Third-order nonlinear optical properties of thin sputtered gold films

被引:56
作者
Xenogiannopoulou, E.
Aloukos, P.
Couris, S. [1 ]
Kaminska, E.
Piotrowska, A.
Dynowska, E.
机构
[1] Univ Patras, Dept Phys, Patras 26500, Greece
[2] Fdn Res & Technol Hellas, FORTH, Inst Chem Engn & High Temp Chem Proc, ICEHT, Patras 26504, Greece
[3] Inst Electr Mat Technol, Warsaw, Poland
[4] Polish Acad Sci, Inst Phys, Warsaw, Poland
关键词
Au films; third-order susceptibility; nonlinear optical properties; optical Kerr effect; Z-scan;
D O I
10.1016/j.optcom.2007.02.059
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Au films of thickness ranging between 5 and 52 nm were prepared by sputtering on quartz substrates and their third-order nonlinear optical response was investigated by Optical Kerr effect (OKE) and Z-scan techniques using 532 nm, 35 ps laser pulses. All prepared films were characterized by XRD, AFM and UV-VIS-NIR spectrophotometry while their third-order susceptibility chi((3)) was measured and found to be of the order of 10(-9) esu. The real and imaginary parts of the third-order susceptibility were found in very good agreement with experimental results and theoretical predictions reported by Smith et al. [D.D. Smith, Y. Yoon, R.W. Boyd, Y.K. Cambell, L.A. Baker, R.M. Crooks, M. George, J. Appl. Phys. 86 (1999) 6200]. (c) 2007 Elsevier B.V. All rights reserved.
引用
收藏
页码:217 / 222
页数:6
相关论文
共 22 条
[1]  
Boyd R.W., 1992, NONLINEAR OPTICS, P166
[2]  
Chopra K. L., 1969, Thin Films Phenomena
[3]   CONCENTRATION AND WAVELENGTH DEPENDENCE OF THE EFFECTIVE 3RD-ORDER SUSCEPTIBILITY AND OPTICAL LIMITING OF C-60 IN TOLUENE SOLUTION [J].
COURIS, S ;
KOUDOUMAS, E ;
RUTH, AA ;
LEACH, S .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 1995, 28 (20) :4537-4554
[4]  
Cullity B., 1978, ELEMENTS XRAY DIFFRA
[5]   Characterization of optical and nonlinear optical properties of silver nanoparticles prepared by laser ablation in various liquids [J].
Ganeev, RA ;
Baba, M ;
Ryasnyansky, AI ;
Suzuki, M ;
Kuroda, H .
OPTICS COMMUNICATIONS, 2004, 240 (4-6) :437-448
[6]   THE OPTICAL KERR EFFECT IN SMALL METAL PARTICLES AND METAL COLLOIDS - THE CASE OF GOLD [J].
HACHE, F ;
RICARD, D ;
FLYTZANIS, C ;
KREIBIG, U .
APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING, 1988, 47 (04) :347-357
[7]   OPTICAL KERR EFFECT IN LIQUIDS [J].
HO, PP ;
ALFANO, RR .
PHYSICAL REVIEW A, 1979, 20 (05) :2170-2187
[8]   Influence of size effect and sputtering conditions on the crystallinity and optical properties of ZnO thin films [J].
Kapustianyk, V. ;
Turko, B. ;
Kostruba, A. ;
Sofiani, Z. ;
Derkowska, B. ;
Dabos-Seignon, S. ;
Barwinski, B. ;
Eliyashevskyi, Yu. ;
Sahraoui, B. .
OPTICS COMMUNICATIONS, 2007, 269 (02) :346-350
[9]   Optical characteristics of gold nanoparticle-doped multilayer thin film [J].
Liao, HB ;
Lu, WX ;
Yu, SW ;
Wen, WJ ;
Wong, GKL .
JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS, 2005, 22 (09) :1923-1926
[10]   Large third-order nonlinear optical susceptibility of Au-Al2O3 composite films near the resonant frequency [J].
Liao, HB ;
Xiao, RF ;
Fu, JS ;
Wong, GKL .
APPLIED PHYSICS B-LASERS AND OPTICS, 1997, 65 (4-5) :673-676