Multiexcitonic two-state lasing in a CdSe nanocrystal laser

被引:68
作者
Chan, Y [1 ]
Caruge, JM [1 ]
Snee, PT [1 ]
Bawendi, MG [1 ]
机构
[1] MIT, Dept Chem, Cambridge, MA 02139 USA
基金
美国国家科学基金会; 德国科学基金会;
关键词
D O I
10.1063/1.1795368
中图分类号
O59 [应用物理学];
学科分类号
摘要
We report simultaneous amplified spontaneous emission from two different multiexcitonic transitions -1S(e)-1S(3/2) and 1P(e)-1P(3/2)(-) of colloidal CdSe nanocrystals (NCs) stabilized in high volume fraction in titania matrices. Two-state lasing from both multiexcitonic transitions is achieved in a surface-emitting distributed feedback CdSe NC laser. Variable stripe length measurements show that the gain from the 1P(e)-1P(3/2) transition is approximately twice that of the -1S(e)-1S(3/2) transition for 4.2 nm radius CdSe/ZnS core-shell NCs. (C) American Institute of Physics.
引用
收藏
页码:2460 / 2462
页数:3
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