Instrumentation, data evaluation and quantification in on-line aerosol mass spectrometry

被引:58
作者
Hinz, Klaus-Peter [1 ]
Spengler, Bernhard [1 ]
机构
[1] Univ Giessen, Inst Inorgan & Analyt Chem, D-35392 Giessen, Germany
来源
JOURNAL OF MASS SPECTROMETRY | 2007年 / 42卷 / 07期
关键词
chemical composition; mass spectrometry; on-line particle analysis; atmospheric aerosols; clustering algorithms;
D O I
10.1002/jms.1262
中图分类号
Q5 [生物化学];
学科分类号
071010 ; 081704 ;
摘要
On-line micro- and nanoparticle mass spectrometry has evolved into a prominent analytical method for the characterization of airborne particles, particle populations and aerosols over the recent years, driven by essential developments in instrumentation, data evaluation and validation. In this tutorial, the fundamental aspects of the technology and methodology for qualitative and quantitative on-line aerosol particle analysis are discussed. Specific properties of the on-line mass spectrometric instrumentation for particle analysis are described, combined with a discussion of basic differences of the instruments and demands for future improvements of instruments and data analysis techniques. Optimized technology and methodology in particle analysis is expected to lead to essential growth of the knowledge and to quality improvement of the description of atmospheric processes and health effects in the future. Copyright (c) 2007 John Wiley & Sons, Ltd.
引用
收藏
页码:843 / 860
页数:18
相关论文
共 165 条
[1]   Quantitative sampling using an Aerodyne aerosol mass spectrometer - 1. Techniques of data interpretation and error analysis [J].
Allan, JD ;
Jimenez, JL ;
Williams, PI ;
Alfarra, MR ;
Bower, KN ;
Jayne, JT ;
Coe, H ;
Worsnop, DR .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2003, 108 (D3)
[2]   A generalised method for the extraction of chemically resolved mass spectra from aerodyne aerosol mass spectrometer data [J].
Allan, JD ;
Delia, AE ;
Coe, H ;
Bower, KN ;
Alfarra, MR ;
Jimenez, JL ;
Middlebrook, AM ;
Drewnick, F ;
Onasch, TB ;
Canagaratna, MR ;
Jayne, JT ;
Worsnop, DR .
JOURNAL OF AEROSOL SCIENCE, 2004, 35 (07) :909-922
[3]   MASS-SPECTROMETRIC ANALYZER FOR INDIVIDUAL AEROSOL-PARTICLES [J].
ALLEN, J ;
GOULD, RK .
REVIEW OF SCIENTIFIC INSTRUMENTS, 1981, 52 (06) :804-809
[4]  
ALLEN J, 1986, PHYS CHEM CHARACTERI, pCH6
[5]   Particle detection efficiencies of aerosol time of flight mass spectrometers under ambient sampling conditions [J].
Allen, JO ;
Fergenson, DP ;
Gard, EE ;
Hughes, LS ;
Morrical, BD ;
Kleeman, MJ ;
Gross, DS ;
Gälli, ME ;
Prather, KA ;
Cass, GR .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2000, 34 (01) :211-217
[6]   Instrument busy time and mass measurement using aerosol time-of-flight mass spectrometry [J].
Allen, Jonathan O. ;
Bhave, Prakash V. ;
Whiteaker, Jeffrey R. ;
Prather, Kimberly A. .
AEROSOL SCIENCE AND TECHNOLOGY, 2006, 40 (08) :615-626
[7]   The pathophysiology of cigarette C-V smoking and cardiovascular disease - An update [J].
Ambrose, JA ;
Barua, RS .
JOURNAL OF THE AMERICAN COLLEGE OF CARDIOLOGY, 2004, 43 (10) :1731-1737
[8]   Climate forcing by aerosols - a hazy picture [J].
Anderson, TL ;
Charlson, RJ ;
Schwartz, SE ;
Knutti, R ;
Boucher, O ;
Rodhe, H ;
Heintzenberg, J .
SCIENCE, 2003, 300 (5622) :1103-1104
[9]  
[Anonymous], 2006, MANAGEMENT MULTIDRUG
[10]  
APPEL BR, 1993, AEROSOL MEASUREMENT, pCH12