Concentrations of 137Cs, 239,240Pu and 210Pb in sediment samples from the Pechora Sea and biological samples from the Ob, Yenisey Rivers and Kara Sea

被引:15
作者
Baskaran, M [1 ]
Asbill, S
Schwantes, J
Santschi, P
Champ, MA
Brooks, JM
Adkinson, D
Makeyev, V
机构
[1] Wayne State Univ, Dept Geol, Detroit, MI 48202 USA
[2] Texas A&M Univ, Dept Oceanog, Galveston, TX 77551 USA
[3] Geochem & Environm Res Grp, College Stn, TX 77845 USA
[4] Res Inst Nat Conservat Arctic & North, St Petersburg, Russia
关键词
plutonium; radiocesium; radioactivity; arctic contamination; Pechora Sea; Kara Sea;
D O I
10.1016/S0025-326X(00)00078-3
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
We have measured the concentrations of Pu-239.240, Pu-238, Pb-210, and Cs-137 in biological samples (5 isopods, 10 bivalves, 2 amphipods, 2 mussell, 1 fish fat, 6 fish liver and 2 worm tubes) from the Ob and Yenisey Rivers and Kara Sea and sediment samples from the Pechora Sea of the Russian Arctic. Mean concentrations of Cs-137 and Pu-239.240 in bivalves on which measurable concentrations were found are slightly higher than the values reported for the east, west and Gulf coasts of US. The mean concentrations of Cs-137 and Pu-239.240 in 27 surficial sediment samples from the Pechora Sea are lower than the corresponding values from the Ob and Yenisey Rivers and Kara Sea, The Pu-238/ Pu-239,Pu-240 activity ratios on 16 of these sediment samples varied between 0.015 and 0.056, The best-fit line between the concentrations of Pu-238 and Pu-239.240 yielded a mean Pu-238/Pu-239,Pu-240 activity ratio of 0.035, suggesting that most of this Pu is derived from global fallout and that there is virtually no detectable input of Pu from either the European nuclear effluents, close-in fallout from the nuclear test sites or from the dumped nuclear reactors in the Kara Sea or adjoining marine systems. (C) 2000 Elsevier Science Ltd. All rights reserved.
引用
收藏
页码:830 / 838
页数:9
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