Pinning of size-selected Ag clusters on graphite surfaces

被引:93
作者
Carroll, SJ [1 ]
Pratontep, S
Streun, M
Palmer, RE
Hobday, S
Smith, R
机构
[1] Univ Birmingham, Sch Phys & Astron, Nanoscale Phys Res Lab, Birmingham B15 2TT, W Midlands, England
[2] Univ Loughborough, Sch Math & Phys, Loughborough LE11 3TU, Leics, England
关键词
D O I
10.1063/1.1322657
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We have explored the deposition of size-selected Ag-N(+) clusters (N=50-200) onto the graphite surface (at room temperature) over the impact energy range of 250-2500 eV, via a combination of scanning tunneling microscopy experiments and molecular dynamics simulations. We show that the clusters are pinned to the surface when the impact energy exceeds a critical value, which is proportional to the cluster size, N, via the formation of a point defect at the impact site. This prevents lateral diffusion of the clusters even at room temperature. (C) 2000 American Institute of Physics. [S0021-9606(00)71742-9].
引用
收藏
页码:7723 / 7727
页数:5
相关论文
共 20 条
[1]  
ACKLAND G, 1987, PHILOS MAG A, V56, P736
[2]   Diffusion and aggregation of large antimony and gold clusters deposited on graphite [J].
Bardotti, L ;
Jensen, P ;
Hoareau, A ;
Treilleux, M ;
Cabaud, B ;
Perez, A ;
Aires, FCS .
SURFACE SCIENCE, 1996, 367 (03) :276-292
[3]   EMPIRICAL POTENTIAL FOR HYDROCARBONS FOR USE IN SIMULATING THE CHEMICAL VAPOR-DEPOSITION OF DIAMOND FILMS [J].
BRENNER, DW .
PHYSICAL REVIEW B, 1990, 42 (15) :9458-9471
[4]   Controlled deposition of size-selected silver nanoclusters [J].
Bromann, K ;
Felix, C ;
Brune, H ;
Harbich, W ;
Monot, R ;
Buttet, J ;
Kern, K .
SCIENCE, 1996, 274 (5289) :956-958
[5]   Self-organized growth of nanostructure arrays on strain-relief patterns [J].
Brune, H ;
Giovannini, M ;
Bromann, K ;
Kern, K .
NATURE, 1998, 394 (6692) :451-453
[6]   Deposition and diffusion of size-selected (Ag400+) clusters on a stepped graphite surface [J].
Carroll, SJ ;
Palmer, RE ;
Mulheran, PA ;
Hobday, S ;
Smith, R .
APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING, 1998, 67 (06) :613-619
[7]   The impact of size-selected ag clusters on graphite: An STM study [J].
Carroll, SJ ;
Weibel, P ;
vonIssendorff, B ;
Kuipers, L ;
Palmer, RE .
JOURNAL OF PHYSICS-CONDENSED MATTER, 1996, 8 (41) :L617-L624
[8]   Energetic impact of size-selected metal cluster ions on graphite [J].
Carroll, SJ ;
Hall, SG ;
Palmer, RE ;
Smith, R .
PHYSICAL REVIEW LETTERS, 1998, 81 (17) :3715-3718
[9]   Trapping of size-selected Ag clusters at surface steps [J].
Carroll, SJ ;
Seeger, K ;
Palmer, RE .
APPLIED PHYSICS LETTERS, 1998, 72 (03) :305-307
[10]  
CARROLL SJ, 1999, THESIS U BIRMINGHAM