Mixed quantum-thermal relaxation in Mn12 acetate molecules

被引:150
作者
Fort, A
Rettori, A
Villain, J
Gatteschi, D
Sessoli, R
机构
[1] Univ Florence, Dipartimento Fis, I-50125 Florence, Italy
[2] Ist Nazl Fis Nucl, I-50125 Florence, Italy
[3] CEA, Dept Rech Fondamentale Mat Condensee, F-38054 Grenoble, France
[4] CNRS, Ctr Rech Tres Basses Temp, F-38042 Grenoble, France
[5] Univ Florence, Dipartimento Chim, I-50144 Florence, Italy
关键词
D O I
10.1103/PhysRevLett.80.612
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We present a theoretical and experimental study of the magnetic field dependence of the relaxation of the Mn12O12 acetate compound. For T greater than or equal to 2 K the molecule which starts from the by means of thermal mechanism, while the remaining barrier is crossed by tunneling. This mired quantum-thermal mechanism shows a critical dependence of the relaxation time with respect to the external magnetic field.
引用
收藏
页码:612 / 615
页数:4
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