Universal attosecond response to the removal of an electron

被引:162
作者
Breidbach, J [1 ]
Cederbaum, LS [1 ]
机构
[1] Heidelberg Univ, Inst Phys Chem, D-69120 Heidelberg, Germany
关键词
D O I
10.1103/PhysRevLett.94.033901
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
When an electron is suddenly removed, a universal response of the system is shown to occur on an attosecond (10(-18) s) time scale. During this response time, which lasts about 50 attoseconds, the density of the created hole changes in a characteristic way. Explicit examples are shown. The results are analyzed in terms of the eigenstates of the residual ion and related to the filling of the exchange-correlation hole associated with the electron in the ground state of the system by the remaining electrons.
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页数:4
相关论文
共 12 条
[1]   Migration of holes: Formalism, mechanisms, and illustrative applications [J].
Breidbach, J ;
Cederbaum, LS .
JOURNAL OF CHEMICAL PHYSICS, 2003, 118 (09) :3983-3996
[2]   CORRELATION-EFFECTS IN THE IONIZATION OF MOLECULES - BREAKDOWN OF THE MOLECULAR-ORBITAL PICTURE [J].
CEDERBAUM, LS ;
DOMCKE, W ;
SCHIRMER, J ;
VONNIESSEN, W .
ADVANCES IN CHEMICAL PHYSICS, 1986, 65 :115-159
[3]   Time-resolved atomic inner-shell spectroscopy [J].
Drescher, M ;
Hentschel, M ;
Kienberger, R ;
Uiberacker, M ;
Yakovlev, V ;
Scrinzi, A ;
Westerwalbesloh, T ;
Kleineberg, U ;
Heinzmann, U ;
Krausz, F .
NATURE, 2002, 419 (6909) :803-807
[4]  
Fetter A. L., 2003, Quantum Theory of Many-Particle Systems
[5]  
HUFNER S, 2002, PHOTOELECTRON SPECTR
[6]  
Mahan G. D., 2013, Many-Particle Physics
[7]  
MEHLDORN W, 1982, ENCY PHYS CORPUSCLES
[8]   Ionization of helium in the attosecond equivalent light pulse of 1 GeV/Nucleon U92+ projectiles [J].
Moshammer, R ;
Schmitt, W ;
Ullrich, J ;
Kollmus, H ;
Cassimi, A ;
Dorner, R ;
Jagutzki, O ;
Mann, R ;
Olson, RE ;
Prinz, HT ;
SchmidtBocking, H ;
Spielberger, L .
PHYSICAL REVIEW LETTERS, 1997, 79 (19) :3621-3624
[9]   Probing molecular dynamics with attosecond resolution using correlated wave packet pairs [J].
Niikura, H ;
Légaré, F ;
Hasbani, R ;
Ivanov, MY ;
Villeneuve, DM ;
Corkum, PB .
NATURE, 2003, 421 (6925) :826-829
[10]  
Parr R. G., 1989, INT J QUANTUM CHEM, V47, P101