Characteristics and provenance of dustfall during an unusual floating dust event

被引:40
作者
Lue, Y. L. [1 ,2 ]
Liu, L. Y. [1 ,2 ,3 ]
Hu, X. [1 ,2 ]
Wang, L. [2 ,4 ]
Guo, L. L. [1 ,2 ]
Gao, S. Y. [1 ,2 ,3 ]
Zhang, X. X. [1 ,2 ]
Tang, Y. [1 ,2 ]
Qu, Z. Q. [1 ,2 ]
Cao, H. W. [1 ,2 ]
Jia, Z. J. [1 ,2 ]
Xu, H. Y. [1 ,2 ]
Yang, Y. Y. [1 ,2 ]
机构
[1] Beijing Normal Univ, Acad Disaster Reduct & Emergency Management, Beijing 100875, Peoples R China
[2] Beijing Normal Univ, Key Lab Environm Change & Nat Disaster, Minist Educ, Beijing 100875, Peoples R China
[3] Beijing Normal Univ, State Key Lab Earth Surface Proc & Resource Ecol, Beijing 100875, Peoples R China
[4] Capital Normal Univ, Coll Environm Resources & Tourism, Beijing 100048, Peoples R China
关键词
Floating dust; Morphology; Size distribution; Elemental composition; Dust provenance; ASIAN DUST; CHEMICAL-COMPOSITION; SIZE DISTRIBUTION; LOESS PLATEAU; TRACE-METALS; PARTICLES; STORM; CHINA; TRANSPORT; JAPAN;
D O I
10.1016/j.atmosenv.2010.06.027
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
This study aims to investigate the characteristics, provenance, and particle-related pollution of an intense dustfall event that occurred in Beijing on 16-17 April 2006. Satellite images reveal that the aeolian dust originated in northeastern Alxa League of Inner Mongolia and passed southeastward across northern Ningxia, middle Inner Mongolia, northern Shaanxi, Shanxi, and Hebei provinces. The dust then moved out of continental China in the vicinity of Beijing and Tianjin. The floating dust led to severe air pollution in Huhhot, Datong, and Beijing. We measured dustfall by collecting dust samples, investigated particle morphology, and calculated the mass medium diameter (MMD) of the dustfall using a scanning electron microscope (SEM). Major elements and mineral content of the dust particles were determined by electron probe and powder X-ray diffractometer, respectively. The relative abundance of dustfall during this event was 12.5-15.0 gm(-2), making up about 10% of the total annual dustfall in Beijing. Dustfall amounted to 205 thousand tons in Beijing, the largest amount observed in recent years. The dust particles were mostly angular, subangular and subrounded in morphology, and the MMD was nearly 12 pm. Particles <10 mu m accounted for 54.7% by number, but fine sand particles (larger than 50 mu m) made up 53.7% by volume. Particles with diameters larger than 20 mu m made up of the predominant volume of the samples (90.35%). Hence, this dustfall event was characterized by a high content of fine sand and coarse silt particles. The principal elements in the dust particles were C, O, Si, Al, Fe, and Ca, whereas the major minerals were quartz, Na-feldspar, calcite, and clay minerals. (C) 2010 Elsevier Ltd. All rights reserved.
引用
收藏
页码:3477 / 3484
页数:8
相关论文
共 59 条
[1]   Global air quality and pollution [J].
Akimoto, H .
SCIENCE, 2003, 302 (5651) :1716-1719
[2]  
[Anonymous], J DESERT RES
[3]   Characterization of Asian Dust during ACE-Asia [J].
Arimoto, R. ;
Kim, Y. J. ;
Kim, Y. P. ;
Quinn, P. K. ;
Bates, T. S. ;
Anderson, T. L. ;
Gong, S. ;
Uno, I. ;
Chin, M. ;
Huebert, B. J. ;
Clarke, A. D. ;
Shinozuka, Y. ;
Weber, R. J. ;
Anderson, J. R. ;
Guazzotti, S. A. ;
Sullivan, R. C. ;
Sodeman, D. A. ;
Prather, K. A. ;
Sokolik, I. N. .
GLOBAL AND PLANETARY CHANGE, 2006, 52 (1-4) :23-56
[4]  
BERGAMETTI G, 1989, NATO ADV SCI I C-MAT, V282, P227
[5]   Particle inhalability at low wind speeds [J].
Brown, JS .
INHALATION TOXICOLOGY, 2005, 17 (14) :831-837
[6]  
Chen L. H., 1986, APPL SCANNING ELECT, P72
[7]   Effects of Asian dust storm events on daily mortality in Taipei, Taiwan [J].
Chen, YS ;
Sheen, PC ;
Chen, ER ;
Liu, YK ;
Wu, TN ;
Yang, CY .
ENVIRONMENTAL RESEARCH, 2004, 95 (02) :151-155
[8]   Chemical composition and source signature of spring aerosol in Seoul, Korea [J].
Choi, JC ;
Lee, M ;
Chun, Y ;
Kim, J ;
Oh, S .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2001, 106 (D16) :18067-18074
[9]   Characteristic number size distribution of aerosol during Asian dust period in Korea [J].
Chun, Y ;
Kim, J ;
Choi, JC ;
Boo, KO ;
Oh, SN ;
Lee, M .
ATMOSPHERIC ENVIRONMENT, 2001, 35 (15) :2715-2721
[10]   Synopsis, transport, and physical characteristics of Asian dust in Korea [J].
Chun, YS ;
Boo, KO ;
Kim, J ;
Park, SU ;
Lee, M .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2001, 106 (D16) :18461-18469