Mosaic multistate scenario versus one-state description of supercooled liquids

被引:80
作者
Cavagna, Andrea
Grigera, Tomas S.
Verrocchio, Paolo
机构
[1] CNR, INFM, ISC, Inst Stat Mech & Complex, I-00185 Rome, Italy
[2] Natl Univ La Plata, INIFTA, RA-1900 La Plata, Argentina
[3] Natl Univ La Plata, Fac Ciencias Exactas, Dept Fis, RA-1900 La Plata, Argentina
[4] Consejo Nacl Invest Cient & Tecn, Buenos Aires, DF, Argentina
[5] Univ Trent, Dipartimento Fis, I-38050 Trento, Italy
[6] Univ Roma La Sapienza, CNR, INFM, SOFT, I-00185 Rome, Italy
[7] BIFI, Inst Biocomputac & Fis Sistemas Complejos, Zaragoza, Spain
关键词
D O I
10.1103/PhysRevLett.98.187801
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
According to the mosaic scenario, relaxation in supercooled liquids is ruled by two competing mechanisms: surface tension, opposing the creation of local excitations, and entropy, providing the drive to the configurational rearrangement of a given region. We test this scenario through numerical simulations well below the Mode Coupling temperature. For an equilibrated configuration, we freeze all the particles outside a sphere and study the thermodynamics of this sphere. The frozen environment acts as a pinning field. Measuring the overlap between the unpinned and pinned equilibrium configurations of the sphere, we can see whether it has switched to a different state. We do not find any clear evidence of the mosaic scenario. Rather, our results seem compatible with the existence of a single (liquid) state. However, we find evidence of a growing static correlation length, apparently unrelated to the mosaic one.
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页数:4
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