Near-field optical imaging using metal tips illuminated by higher-order Hermite-Gaussian beams

被引:224
作者
Novotny, L [1 ]
Sánchez, EJ [1 ]
Xie, XS [1 ]
机构
[1] Pacific NW Lab, Environm Mol Sci Lab, Richland, WA 99352 USA
关键词
near-field optics; single molecule detection; fluorescence imaging; nonlinear optics; nanotechnology;
D O I
10.1016/S0304-3991(97)00077-6
中图分类号
TH742 [显微镜];
学科分类号
摘要
We propose a new scheme for high-resolution near-field optical imaging. The method relies on the highly enhanced fields at sharp metal tips under laser illumination. These fields are laterally confined to the tip size and can be used to locally excite the sample surface. Illumination along the tip axis with a higher-order beam mode (Hermite-Gaussian(1,0) mode) and detection of nonlinear responses (two-photon fluorescence, generation of second/third harmonics) ensure sufficient background discrimination. We outline the theory of laser beams beyond the paraxial approximation and investigate the electromagnetic fields for the proposed scheme. (C) 1998 Elsevier Science B.V. All rights reserved.
引用
收藏
页码:21 / 29
页数:9
相关论文
共 24 条
[1]   5TH-ORDER CORRECTED ELECTROMAGNETIC-FIELD COMPONENTS FOR A FUNDAMENTAL GAUSSIAN-BEAM [J].
BARTON, JP ;
ALEXANDER, DR .
JOURNAL OF APPLIED PHYSICS, 1989, 66 (07) :2800-2802
[2]   NEAR-FIELD OPTICS - MICROSCOPY, SPECTROSCOPY, AND SURFACE MODIFICATION BEYOND THE DIFFRACTION LIMIT [J].
BETZIG, E ;
TRAUTMAN, JK .
SCIENCE, 1992, 257 (5067) :189-195
[3]   SINGLE MOLECULES OBSERVED BY NEAR-FIELD SCANNING OPTICAL MICROSCOPY [J].
BETZIG, E ;
CHICHESTER, RJ .
SCIENCE, 1993, 262 (5138) :1422-1425
[4]   ACCELERATION OF PARTICLES BY AN ASYMMETRIC HERMITE-GAUSSIAN LASER-BEAM [J].
BOCHOVE, EJ ;
MOORE, GT ;
SCULLY, MO .
PHYSICAL REVIEW A, 1992, 46 (10) :6640-6653
[5]   NEAR-FIELD OPTICS - MICROSCOPY WITH NANOMETER-SIZE FIELDS [J].
DENK, W ;
POHL, DW .
JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B, 1991, 9 (02) :510-513
[6]   NEAR-FIELD FLUORESCENCE IMAGING AND FLUORESCENCE LIFETIME MEASUREMENT OF LIGHT-HARVESTING COMPLEXES IN INTACT PHOTOSYNTHETIC MEMBRANES [J].
DUNN, RC ;
HOLTOM, GR ;
METS, L ;
XIE, XS .
JOURNAL OF PHYSICAL CHEMISTRY, 1994, 98 (12) :3094-3098
[7]   THIN-FILM NANOPROCESSING BY LASER STM COMBINATION [J].
GORBUNOV, AA ;
POMPE, W .
PHYSICA STATUS SOLIDI A-APPLICATIONS AND MATERIALS SCIENCE, 1994, 145 (02) :333-338
[8]   A SCALAR REPRESENTATION OF ELECTROMAGNETIC FIELDS [J].
GREEN, HS ;
WOLF, E .
PROCEEDINGS OF THE PHYSICAL SOCIETY OF LONDON SECTION A, 1953, 66 (408) :1129-1137
[9]  
HAFNER C, 1990, GEN MULTIPLE MULTIPO
[10]  
HAUPT C, 1993, P SOC PHOTO-OPT INS, V1983, P658