Spatial distribution and interannual variation of surface PM10 concentrations over eighty-six Chinese cities

被引:132
作者
Qu, W. J. [1 ,2 ]
Arimoto, R. [3 ]
Zhang, X. Y. [2 ]
Zhao, C. H. [1 ]
Wang, Y. Q. [2 ]
Sheng, L. F. [1 ]
Fu, G. [1 ]
机构
[1] Ocean Univ China, Phys Oceanog Lab, Ocean Atmosphere Interact & Climate Lab, Dept Marine Meteorol,Coll Phys & Environm Oceanog, Qingdao 266100, Peoples R China
[2] Chinese Acad Metrol Sci, China Meteorol Adm, Key Lab Atmospher Chem, CAWAS, Beijing 100081, Peoples R China
[3] New Mexico State Univ, Carlsbad Environm Monitoring & Res Ctr, Carlsbad, NM USA
基金
美国国家科学基金会;
关键词
AEROSOL OPTICAL DEPTH; PARTICULATE AIR-POLLUTION; LONG-TERM TREND; CHEMICAL CHARACTERISTICS; ATMOSPHERIC AEROSOL; EASTERN CHINA; DELTA REGION; BLACK CARBON; DUST AEROSOL; PM2.5;
D O I
10.5194/acp-10-5641-2010
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The spatial distribution of the aerosols over 86 Chinese cities was reconstructed from air pollution index (API) records for summer 2000 to winter 2006. PM10 ( particulate matter <= 10 mu m) mass concentrations were calculated for days when PM10 was the principal pollutant, these accounted for 91.6% of the total 150 428 recorded days. The 83 cities in mid-eastern China (100 degrees E to 130 degrees E) were separated into three latitudinal zones using natural landscape features as boundaries. Areas with high PM10 level in northern China (127 to 192 mu g m(-3)) included Urumchi, Lanzhou-Xining, Weinan-Xi'an, Taiyuan-Datong-Yangquan-Changzhi, Pingdingshan-Kaifeng, Beijing-Tianjin-Shijiazhuang, Jinan, and Shenyang-Anshan-Fushun; in the middle zone, high PM10 (119-147 mu g m(-3)) occurred at Chongqing-Chengdu-Luzhou, Changsha-Wuhan, and Nanjing-Hangzhou; in the southern zone, only four cities (Qujing, Guiyang, Guangzhou and Shaoguan) showed PM10 concentration > 80 mu g m(-3). The median PM10 concentration decreased from 108 mu g m(-3) for the northern cities to 95 mu g m(-3) and 55 mu g m(-3) for the middle and southern zones, respectively. PM10 concentration and the APIs both exhibited wintertime maxima, summertime minima, and the second highest values in spring. PM10 showed evidence for a decreasing trend for the northern cities while in the other zones urban PM10 levels fluctuated, but showed no obvious change over time. The spatial distribution of PM10 was compared with the emissions, and the relationship between the surface PM10 concentration and the aerosol optical depth (AOD) was also discussed.
引用
收藏
页码:5641 / 5662
页数:22
相关论文
共 89 条
[1]  
[Anonymous], CHIN STAT YB 2005
[2]   Measurements of gaseous HONO, HNO3,SO2, HCl, NH3, particulate sulfate and PM2.5 in New York, NY [J].
Bari, A ;
Ferraro, V ;
Wilson, LR ;
Luttinger, D ;
Husain, L .
ATMOSPHERIC ENVIRONMENT, 2003, 37 (20) :2825-2835
[3]   Source apportionment of PM10 in six cities of northern China [J].
Bi, Xiaohui ;
Feng, Yinchang ;
Wu, Jianhui ;
Wang, Yuqiu ;
Zhu, Tan .
ATMOSPHERIC ENVIRONMENT, 2007, 41 (05) :903-912
[4]   Near-real time retrieval of tropospheric NO2 from OMI [J].
Boersma, K. F. ;
Eskes, H. J. ;
Veefkind, J. P. ;
Brinksma, E. J. ;
Van der A, R. J. ;
Sneep, M. ;
van den Oord, G. H. J. ;
Levelt, P. F. ;
Stammes, P. ;
Gleason, J. F. ;
Bucsela, E. J. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2007, 7 (08) :2103-2118
[5]   Characteristics of carbonaceous aerosol in Pearl River Delta Region, China during 2001 winter period [J].
Cao, JJ ;
Lee, SC ;
Ho, KF ;
Zhang, XY ;
Zou, SC ;
Fung, K ;
Chow, JC ;
Watson, JG .
ATMOSPHERIC ENVIRONMENT, 2003, 37 (11) :1451-1460
[6]   Air pollution in mega cities in China [J].
Chan, Chak K. ;
Yao, Xiaohong .
ATMOSPHERIC ENVIRONMENT, 2008, 42 (01) :1-42
[7]   CLIMATE FORCING BY ANTHROPOGENIC AEROSOLS [J].
CHARLSON, RJ ;
SCHWARTZ, SE ;
HALES, JM ;
CESS, RD ;
COAKLEY, JA ;
HANSEN, JE ;
HOFMANN, DJ .
SCIENCE, 1992, 255 (5043) :423-430
[8]   Particulate air pollution in Lanzhou China [J].
Chu, Peter C. ;
Chen, Yuchun ;
Lu, Shihua ;
Li, Zhenchao ;
Lu, Yaqiong .
ENVIRONMENT INTERNATIONAL, 2008, 34 (05) :698-713
[9]  
*CLIM SOURC INC, PRISM 1961 1990 MEAN
[10]   Airborne analysis of the Los Angeles aerosol [J].
Collins, DR ;
Jonsson, HH ;
Liao, H ;
Flagan, RC ;
Seinfeld, JH ;
Noone, KJ ;
Hering, SV .
ATMOSPHERIC ENVIRONMENT, 2000, 34 (24) :4155-4173