Cl-NMR study on field-induced magnetic order in quasi-one-dimensional antiferromagnet (CH3)2CHNH3CUCl3

被引:7
作者
Saito, T. [1 ]
Inoue, H. [1 ]
Tonisi, J. [1 ]
Oosawa, A. [1 ]
Goto, T. [1 ]
Sasaki, T. [2 ]
Kobayasi, N. [2 ]
Awaji, S. [2 ]
Watanabe, K. [2 ]
机构
[1] Sophia Univ, Dept Phys, Chiyoda Ku, Tokyo 102, Japan
[2] Tohoku Univ, Inst Mat Res, Sendai, Miyagi 9808577, Japan
来源
YAMADA CONFERENCE LX ON RESEARCH IN HIGH MAGNETIC FIELDS | 2006年 / 51卷
关键词
D O I
10.1088/1742-6596/51/1/047
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
(CH3)(2)CHNH3CuCl3 is described as the spin ladder system, which is composed of a strong ferromagnetic rung and a weak antiferromagnetic leg. Since the ferromagnetic dimer behaves like S=1 spin, this system can be treated as the S=1 quasi-one-dimensional antiferromagnet spin chain (so-called Haldane chain). Cl-NMR study under high-field up to 17.5T has been carried out in order to investigate the field-induced magnetic order in this system. In the lower field region below 10T, the signals from Cl-sites were observed as sharp NMR lines. These paramagnetic lines showed the split above H-N(red) similar or equal to 12T (T=1.85K), demonstrating the existence of the staggered field due to the field-induced magnetic order. Around H-N, the resonance lines disappeared due to the critical slowing down when the applied magnetic field was perpendicular to the ladder, whereas they did not when the field was nearly parallel to the ladder. These results indicate that the spin dynamics around the field-induced magnetic order is anisotropic in this system.
引用
收藏
页码:203 / +
页数:2
相关论文
共 10 条
[3]   Crossover from S=1/2 to S=1 Haldane state in the ferromagnetic and antiferromagnetic alternating Heisenberg chain system (CH3)2CHNH3CuCl3 observed with EPR at 24 GHz [J].
Manaka, H ;
Yamada, I .
PHYSICAL REVIEW B, 2000, 62 (21) :14279-14286
[4]   Ferromagnetic-dominant alternating Heisenberg chains with ferromagnetic and antiferromagnetic interactions formed in (CH3)(2)CHNH3CuCl3 [J].
Manaka, H ;
Yamada, I ;
Yamaguchi, K .
JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN, 1997, 66 (03) :564-567
[5]   Field-induced magnetic long-range order in the ferromagnetic-antiferromagnetic alternating Heisenberg chain system (CH3)2CHNH3CuCl3 observed by specific heat measurements [J].
Manaka, H ;
Yamada, I ;
Honda, Z ;
Katori, HA ;
Katsumata, K .
JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN, 1998, 67 (11) :3913-3917
[6]   Field-induced magnetization in ferromagnetic and antiferromagnetic alternating Heisenberg chains formed in (CH3)2CHNH3CuCl3 [J].
Manaka, H ;
Yamada, I ;
Mushnikov, NV ;
Goto, T .
JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN, 2000, 69 (03) :675-678
[7]   High-field and high-frequency ESR study of the Haldane state formed in the ferromagnetic and antiferromagnetic alternating Heisenberg chain system (CH3)2CHNH3CuCl3 -: art. no. 144428 [J].
Manaka, H ;
Yamada, I ;
Hagiwara, M ;
Tokunaga, M .
PHYSICAL REVIEW B, 2001, 63 (14)
[8]  
MANAKA H, COMMUNICATION
[9]   Dynamics of composite haldane spin chains in IPA-CuCl3 -: art. no. 047210 [J].
Masuda, T ;
Zheludev, A ;
Manaka, H ;
Regnault, LP ;
Chung, JH ;
Qiu, Y .
PHYSICAL REVIEW LETTERS, 2006, 96 (04)
[10]   THERMOCHROMIC PHASE-TRANSITIONS IN COPPER(II) HALIDE SALTS .1. CRYSTAL-STRUCTURE AND MAGNETIC-RESONANCE STUDIES OF (CH3)2CHNH3CUCL3 [J].
ROBERTS, SA ;
BLOOMQUIST, DR ;
WILLETT, RD ;
DODGEN, HW .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1981, 103 (10) :2603-2610