Midinfrared absorption in YBa2Cu3O6:: Evidence for a failure of spin-wave theory for spin 1/2 in two dimensions

被引:44
作者
Grüninger, M
van der Marel, D
Damascelli, A
Erb, A
Nunner, T
Kopp, T
机构
[1] Univ Geneva, Dept Phys Mat Condensee, CH-1211 Geneva, Switzerland
[2] Univ Groningen, MSC, Solid State Phys Lab, NL-9747 AG Groningen, Netherlands
[3] Univ Augsburg, D-86135 Augsburg, Germany
关键词
D O I
10.1103/PhysRevB.62.12422
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The optical conductivity sigma(omega) of undoped and very low doped YBa2Cu3O6.0 delta is studied in detail in the midinfrared range. We collect experimental evidence for a magnetic origin of the observed absorption. The main resonance peak is well described by a bimagnon-plus-phonon absorption spectrum calculated within spin-wave theory. But spin-wave theory fails to describe further resonances at higher frequencies with significant spectral weight, which grows with both temperature and doping. This underlines the importance of quantum fluctuations for the description of short-wavelength magnetic excitations in a two-dimensional spin-1/2 system.
引用
收藏
页码:12422 / 12426
页数:5
相关论文
共 41 条
[1]   PRESSURE-DEPENDENCE OF THE SUPEREXCHANGE INTERACTION IN ANTIFERROMAGNETIC LA2CUO4 [J].
ARONSON, MC ;
DIERKER, SB ;
DENNIS, BS ;
CHEONG, SW ;
FISK, Z .
PHYSICAL REVIEW B, 1991, 44 (09) :4657-4660
[2]   Resonant two-magnon Raman scattering in cuprate antiferromagnetic insulators [J].
Blumberg, G ;
Abbamonte, P ;
Klein, MV ;
Lee, WC ;
Ginsberg, DM ;
Miller, LL ;
Zibold, A .
PHYSICAL REVIEW B, 1996, 53 (18) :11930-11933
[3]   Superexchange coupling and spin susceptibility spectral weight in undoped monolayer cuprates [J].
Bourges, P ;
Casalta, H ;
Ivanov, AS ;
Petitgrand, D .
PHYSICAL REVIEW LETTERS, 1997, 79 (24) :4906-4909
[4]   COMMON INTERATOMIC POTENTIAL MODEL FOR THE LATTICE-DYNAMICS OF SEVERAL CUPRATES [J].
CHAPLOT, SL ;
REICHARDT, W ;
PINTSCHOVIUS, L ;
PYKA, N .
PHYSICAL REVIEW B, 1995, 52 (10) :7230-7242
[5]   Dispersion of a single hole in an antiferromagnet [J].
Chubukov, AV ;
Morr, DK .
PHYSICAL REVIEW B, 1998, 57 (09) :5298-5311
[6]   RESONANT 2-MAGNON RAMAN-SCATTERING IN ANTIFERROMAGNETIC INSULATORS [J].
CHUBUKOV, AV ;
FRENKEL, DM .
PHYSICAL REVIEW LETTERS, 1995, 74 (15) :3057-3060
[7]   OPTICAL STUDIES OF GAP, EXCHANGE, AND HOPPING ENERGIES IN THE INSULATING CUPRATES [J].
COOPER, SL ;
THOMAS, GA ;
MILLIS, AJ ;
SULEWSKI, PE ;
ORENSTEIN, J ;
RAPKINE, DH ;
CHEONG, SW ;
TREVOR, PL .
PHYSICAL REVIEW B, 1990, 42 (16) :10785-10788
[8]  
DEGRAAF C, COMMUNICATION
[9]   DYNAMICS OF AN S=1/2, ONE-DIMENSIONAL HEISENBERG ANTIFERROMAGNET [J].
ENDOH, Y ;
SHIRANE, G ;
BIRGENEAU, RJ ;
RICHARDS, PM ;
HOLT, SL .
PHYSICAL REVIEW LETTERS, 1974, 32 (04) :170-173
[10]   YBA2CU3O(7-DELTA)-BACUO2-CUO - INVESTIGATIONS ON THE PHASE-DIAGRAM AND GROWTH OF SINGLE-CRYSTALS .2. [J].
ERB, A ;
TRAULSEN, T ;
MULLERVOGT, G .
JOURNAL OF CRYSTAL GROWTH, 1994, 137 (3-4) :487-492