Synthesis, characterisation and HDN activity of iron-vanadium sulphide prepared with the use of a chelating agent

被引:8
作者
Magarelli, M [1 ]
Scott, CE [1 ]
Moronta, D [1 ]
Betancourt, P [1 ]
机构
[1] Cent Univ Venezuela, Fac Ciencias, Escuela Quim, Ctr Catalisis, Caracas, Venezuela
关键词
hydrotreating; vanadium sulphide; iron-vanadium sulphide; chelating agent;
D O I
10.1016/S0920-5861(02)00307-3
中图分类号
O69 [应用化学];
学科分类号
081704 ;
摘要
The influence of the use of ethylenediamine in the preparation of iron-vanadium catalyst for toluene hydrogenation (HYD) and pyridine hydrodenitrogenation (HDN) has been studied. Both HYD and HDN activities increased significantly with Fe incorporation to vanadium sulphide and the beneficial effect of ethylenediamine was shown. Possible explanations for the enhancements in HYD and HDN conversion are discussed. (C) 2002 Elsevier Science B.V. All rights reserved.
引用
收藏
页码:339 / 344
页数:6
相关论文
共 21 条
[1]  
[Anonymous], CATAL TODAY
[2]   CHEMISTRY, THERMODYNAMICS AND KINETICS OF REACTIONS OF SULFUR IN COAL-GAS REACTIONS - REVIEW [J].
ATTAR, A .
FUEL, 1978, 57 (04) :201-212
[3]  
GOBOLOS S, 1987, ACTA CHIM HUNG, V124, P177
[4]   X-RAY ABSORPTION K-EDGES STUDIES OF IRON, VANADIUM AND SULFUR IN HDM CLAY CATALYSTS [J].
GONZALEZJIMENEZ, F ;
BAZIN, D ;
DEXPERT, H ;
VILLAIN, F ;
CONSTANT, H ;
ROSABRUSSIN, M .
PHYSICA B, 1989, 158 (1-3) :215-216
[5]   HYDRODENITROGENATION-SELECTIVE CATALYSTS .1. FE PROMOTED MO/W SULFIDES [J].
HO, TC ;
JACOBSON, AJ ;
CHIANELLI, RR ;
LUND, CRF .
JOURNAL OF CATALYSIS, 1992, 138 (01) :351-363
[6]   PROMOTION EFFECTS IN BULK METAL SULFIDE CATALYSTS [J].
HO, TC ;
CHIANELLI, RR ;
JACOBSON, AJ .
APPLIED CATALYSIS A-GENERAL, 1994, 114 (01) :127-139
[7]   ESR IDENTIFICATION OF VANADIUM SPECIES DEPOSITED ON AL2O3 AND MOS2-AL2O3 CATALYSTS - RELEVANCE TO CATALYTIC DEMETALATION OF VANADYL PORPHYRIN [J].
HUBAUT, R ;
AISSI, CF ;
DEJONGHE, S ;
GRIMBLOT, J .
JOURNAL DE CHIMIE PHYSIQUE ET DE PHYSICO-CHIMIE BIOLOGIQUE, 1991, 88 (09) :1741-1755
[8]   STUDIES OF MOLYBDENUM SULFIDE CATALYSTS - EFFECTS OF PRETREATMENT ON SINTERING, STOICHIOMETRY, AND OXYGEN-CHEMISORPTION [J].
KALTHOD, DG ;
WELLER, SW .
JOURNAL OF CATALYSIS, 1985, 95 (02) :455-464
[9]   CHARACTERIZATION OF FRESH AND LINED-OUT BULK FEMO SULFIDE CATALYSTS [J].
KOO, JY ;
HO, TC .
CATALYSIS LETTERS, 1994, 28 (01) :99-108
[10]  
Luis MA, 1999, STUD SURF SCI CATAL, V127, P203