Violation of the zero-force theorem in the time-dependent Krieger-Li-Iafrate approximation

被引:52
作者
Mundt, Michael [1 ]
Kuemmel, Stephan
van Leeuwen, Robert
Reinhard, Paul-Gerhard
机构
[1] Univ Bayreuth, Inst Phys, D-95440 Bayreuth, Germany
[2] Univ Groningen, Zernike Inst Adv Mat, NL-9747 AG Groningen, Netherlands
[3] Univ Erlangen Nurnberg, Inst Theoret Phys 2, D-91058 Erlangen, Germany
来源
PHYSICAL REVIEW A | 2007年 / 75卷 / 05期
关键词
D O I
10.1103/PhysRevA.75.050501
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We demonstrate that the time-dependent Krieger-Li-Iafrate approximation in combination with the exchange-only functional violates the zero-force theorem. By analyzing the time-dependent dipole moment of Na-5 and Na-9(+), we furthermore show that this can lead to an unphysical self-excitation of the system depending on the system properties and the excitation strength. Analytical aspects, especially the connection between the zero-force theorem and the generalized-translation invariance of the potential, are discussed.
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页数:4
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