Benefits of polarized small-angle neutron scattering on magnetic nanometer scale structure modeling

被引:21
作者
Heinemann, A [1 ]
Wiedenmann, A [1 ]
机构
[1] Hahn Meitner Inst Berlin GmbH, D-14109 Berlin, Germany
关键词
small-angle neutron scattering; polarized neutrons; magnetic scattering; paramagnetic particles; ferrofluid;
D O I
10.1107/S0021889803000207
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Recent use of polarized neutron technique in small-angle scattering (SANS) have led to impressive results in the case of magnetic nanometer-scale structure analysis. In some particular cases this method offers the possibility to survey structure models with the necessary accuracy for the first time. The different cross sections for spin-up and spin-down neutron scattering on magnetic precipitates can be combined with the method of chemical contrast variation. All data fitting using structure models will benefit of that kind of constraints. The analysis of the interference term of nuclear and magnetic scattering respectively enables the extraction of additional information about the composition and magnetization profiles of the samples. Here we place emphasis on the difference of spin-up and spin-down neutron scattering intensities to obtain this information. This technique profits by the clear distinction between magnetic and nonmagnetic scattering contributions and the strong auxiliary conditions for model fitting procedures. Depending on the relative orientations of the external magnetic field, the local magnetization of the precipitates and the scattering vector, significant scattering patterns can be scrutinized. Beside general formulas for some special cases of present experimental interest we exercise the approach to a nontrivial case of data obtained from polarised SANS experiments at the Berlin Neutron Scattering Center (BENSC).
引用
收藏
页码:845 / 849
页数:5
相关论文
共 12 条
[1]  
[Anonymous], 1988, Nonlinear regression analysis and its applications
[2]  
GUREVICH I, 1968, LOW ENERGIE NEUTRON
[3]   A small-angle neutron scattering model for polydisperse spherical particles with diffusion zones and application to soft magnetic metallic glass [J].
Heinemann, A ;
Hermann, H ;
Wiedenmann, A ;
Mattern, N ;
Wetzig, K .
JOURNAL OF APPLIED CRYSTALLOGRAPHY, 2000, 33 :1386-1392
[4]   Structure of magnetite ferrofluids investigated by SANS with polarized neutrons [J].
Kammel, M ;
Hoell, A ;
Wiedenmann, A .
SCRIPTA MATERIALIA, 2001, 44 (8-9) :2341-2345
[5]   Magnetic coupling between the different phases in nanocrystalline Fe-Si-B studied by small angle neutron scattering [J].
Kohlbrecher, J ;
Wiedenmann, A ;
Wollenberger, H .
ZEITSCHRIFT FUR PHYSIK B-CONDENSED MATTER, 1997, 104 (01) :1-4
[6]   POLARIZATION ANALYSIS OF THERMAL-NEUTRON SCATTERING [J].
MOON, RM ;
RISTE, T ;
KOEHLER, WC .
PHYSICAL REVIEW, 1969, 181 (02) :920-&
[7]   DETERMINATION OF FERROFLUID STRUCTURE BY NEUTRON POLARIZATION ANALYSIS [J].
PYNN, R ;
HAYTER, JB ;
CHARLES, SW .
PHYSICAL REVIEW LETTERS, 1983, 51 (08) :710-713
[8]  
RATKOWSKY D., 1983, Nonlinear regression modelling
[9]  
Ratkowsky D.A., 1990, HDB NONLINEAR REGRES
[10]   Small-angle neutron scattering investigations of magnetic nanostructures and interfaces using polarized neutrons [J].
Wiedenmann, A .
PHYSICA B-CONDENSED MATTER, 2001, 297 (1-4) :226-233