Electrodegradation of landfill leachate in a flow electrochemical reactor

被引:135
作者
Moraes, PB [1 ]
Bertazzoli, R [1 ]
机构
[1] Campinas State Univ, Fac Mech Engn, Dept Mat Engn, BR-13083970 Campinas, SP, Brazil
基金
巴西圣保罗研究基金会;
关键词
landfill leachate; electrochemical oxidation; oxide electrodes; effluent degradation; electrolytic treatment; electrochemical flow reactor;
D O I
10.1016/j.chemosphere.2004.09.026
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Sanitary landfills are the major method used today for the disposal and management of municipal solid waste. Decomposition of waste and rainfall generate leachate at the bottom of landfills, causing groundwater contamination. In this study, leachate from a municipal landfill site was treated by electrochemical oxidation in a pilot scale flow reactor, using oxide-coated titanium anode. The experiments were conducted under a constant flow rate of 20001h(-1) and the effect of current density on chemical oxygen demand, total organic carbon, color and ammonium removal was investigated. At a current density of 116.0mAcm(-2) and 180min of processing, the removal rates achieved were 73% for COD, 57% for TOC, 86% for color and 49% for ammonium. The process proved effective in degrading leachate, despite this effluent's usual refractoriness to treatment. (C) 2004 Elsevier Ltd. All rights reserved.
引用
收藏
页码:41 / 46
页数:6
相关论文
共 18 条
[1]  
[Anonymous], 1995, Standard methods for examination of water and waste water, V19th
[2]   Treatment of landfill leachate using activated sludge process and electron-beam radiation [J].
Bae, BU ;
Jung, ES ;
Kim, YR ;
Shin, HS .
WATER RESEARCH, 1999, 33 (11) :2669-2673
[3]   INDIRECT OXIDATION EFFECT IN ELECTROCHEMICAL OXIDATION TREATMENT OF LANDFILL LEACHATE [J].
CHIANG, LC ;
CHANG, JE ;
WEN, TC .
WATER RESEARCH, 1995, 29 (02) :671-678
[4]  
Clement B, 1997, CHEMOSPHERE, V35, P2783, DOI 10.1016/S0045-6535(97)00332-9
[5]   Electrochemical treatment of landfill leachate:: Oxidation at Ti/PbO2 and Ti/SnO2 anodes [J].
Cossu, R ;
Polcaro, AM ;
Lavagnolo, MC ;
Mascia, M ;
Palmas, S ;
Renoldi, F .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1998, 32 (22) :3570-3573
[6]  
Foti G., 1997, CURR TOP ELECTROCHEM, V5, P71
[7]   Improved fenton method to remove recalcitrant organics in landfill leachate [J].
Gau, SH ;
Chang, FS .
WATER SCIENCE AND TECHNOLOGY, 1996, 34 (7-8) :455-462
[8]   BIODEGRADATION AND ADSORPTION IN REFRACTORY LEACHATE TREATMENT BY THE BIOLOGICAL ACTIVATED CARBON FLUIDIZED-BED PROCESS [J].
IMAI, A ;
ONUMA, K ;
INAMORI, Y ;
SUDO, R .
WATER RESEARCH, 1995, 29 (02) :687-694
[9]   Light-enhanced chemical oxidation for tertiary treatment of municipal landfill leachate [J].
Ince, NH .
WATER ENVIRONMENT RESEARCH, 1998, 70 (06) :1161-1169
[10]   The impact of leachate collection on air quality in landfills [J].
James, KJ ;
Stack, MA .
CHEMOSPHERE, 1997, 34 (08) :1713-1721