Correlation of electronic structure and ordered charge and orbital patterns for single-layered manganites in a wide hole-doping range (0≤x≤1)

被引:16
作者
Lee, Y. S. [1 ]
Arima, T.
Onoda, S.
Okimoto, Y.
Tokunaga, Y.
Mathieu, R.
Yu, X. Z.
He, J. P.
Kaneko, Y.
Matsui, Y.
Nagaosa, N.
Tokura, Y.
机构
[1] Japan Sci & Technol Agcy, ERATO, Spin Superstruct Project & Multiferro Project, Tsukuba, Ibaraki 3058562, Japan
[2] Soongsil Univ, Dept Phys, Tsukuba, Ibaraki 156743, Japan
[3] Tohoku Univ, Inst Multidisciplinary Res Adv Mat, Sendai, Miyagi 9808577, Japan
[4] AIST, AIST Tsukuba Cent 4, CERC, Tsukuba, Ibaraki 3058562, Japan
[5] NIMS, Adv Mat Lab, Tsukuba, Ibaraki 3050044, Japan
[6] Univ Tokyo, Dept Appl Phys, Tokyo 1138656, Japan
关键词
D O I
10.1103/PhysRevB.75.144407
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We investigated the doping-dependent evolution of the charge-orbital ordering (CO-OO) phase using optical spectroscopy of a series of single-layer manganites, La1-xSr1+xMnO4 (x=0 and 1) and Pr1-xCa1+xMnO4 (0.3 <= x <= 0.7). We found that the electronic response of the CO-OO phase changes asymmetrically with respect to the addition or removal of e(g) electrons from x=1/2. Especially, low-energy optical spectra depend strongly on the modulation vector of striped phase in a higher doping region (x >= 1/2). This finding highlights the role of the nanoscale structure of e(g) ordering in the electronic property of the striped phase in the layered manganite.
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页数:6
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