Spin-driven Jahn-Teller distortion in a pyrochlore system

被引:236
作者
Yamashita, Y [1 ]
Ueda, K [1 ]
机构
[1] Univ Tokyo, Inst Solid State Phys, Kashiwa, Chiba 2778581, Japan
关键词
D O I
10.1103/PhysRevLett.85.4960
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The ground-state properties of the spin-1 antiferromagnetic Heisenberg model on the comer-sharing tetrahedra, the pyrochlore lattice, are investigated. By breaking up each spin into a pair of 1/2-spins, the problem is reduced to the equivalent one of the spin-1/2 tetrahedral network in analogy with the valence bond solid state in one dimension. The twofold degeneracy of the spin singlets of a tetrahedron is lifted by a Jahn-Teller mechanism, leading to a cubic to tetragonal structural transition, it is proposed that the present mechanism is responsible for the phase transition observed in the spin-1 spinel compounds ZnV2O4 and MgV2O4.
引用
收藏
页码:4960 / 4963
页数:4
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