Experimental verification of the gapless point in the S=1 antiferromagnetic bond alternating chain

被引:59
作者
Hagiwara, M [1 ]
Narumi, Y
Kindo, K
Kohno, M
Nakano, H
Sato, R
Takahashi, M
机构
[1] RIKEN, Inst Phys & Chem Res, Wako, Saitama 35101, Japan
[2] Osaka Univ, KYOKUGEN, Toyonaka, Osaka 560, Japan
[3] Japan Sci & Technol Corp, CREST, Tokyo, Japan
[4] Univ Tokyo, Inst Solid State Phys, Tokyo 106, Japan
关键词
D O I
10.1103/PhysRevLett.80.1312
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Susceptibility and high field magnetization measurements have been performed on powdered samples of [{Ni(333-tet)(mu-N-3)}(n)](ClO4)(n) [333-tet denotes tetraamine N,N'-bis(3-aminopropyl)-1,3-propanediamine]. As the temperature is decreased, the susceptibility exhibits a smooth maximum around 120 K and decreases gradually down to 10 K, and then decreases rapidly. Magnetization up to 50 T at 1.4 K shows no gap in this compound within the experimental accuracy, We have carried our numerical calculations for the S = 1 antiferromagnetic bond alternating chain and obtained very good agreement between experiments and calculations for the alternating ratio alpha = 0.6.
引用
收藏
页码:1312 / 1315
页数:4
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