Antiferromagnetic ordering in the expanded (NH3)Rb3C60 fulleride

被引:5
作者
Arvanitidis, J [1 ]
Papagelis, K
Takenobu, T
Margiolaki, I
Brigatti, K
Prassides, K
Iwasa, Y
Lappas, A
机构
[1] Univ Sussex, Sch Chem Phys & Environm Sci, Brighton BN1 9QJ, E Sussex, England
[2] Tohoku Univ, Mat Res Inst, Aoba Ku, Sendai, Miyagi 9808577, Japan
[3] Japan Sci & Technol Corp, CREST, Kawaguchi 3320012, Japan
[4] Fdn Res & Technol Hellas, Inst Elect Struct & Laser, Iraklion 71110, Greece
关键词
ammoniated alkali fullerides; antiferromagnetic ordering;
D O I
10.1016/S0921-4526(02)01661-7
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
The magnetic behavior of the ammoniated alkali fulleride (NH3)Rb3C60 is studied by means of mu(+) spin relaxation (mu(+) SR) spectroscopy. The observation of a strongly damped oscillating component in the low-temperature zero-field p SR spectra reveals that its ground state is that of an ordered anti ferromagnet. characterized by large spatially inhomogeneous effects. The temperature dependence of the mu(+) spin precession frequency is consistent with that of a ;conventional 3D Heisenberg antiferromagnet (T-N similar to 51 K). The cooling rate of the sample affects sensitively the ordering of the magnetic moments, a behavior that can be attributed to the influence of the orientational order of the fullerene units on the exchange interactions. (C) 2002 Elsevier Science B.V. All rights reserved.
引用
收藏
页码:572 / 576
页数:5
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