Historical (1850-2000) gridded anthropogenic and biomass burning emissions of reactive gases and aerosols: methodology and application

被引：1622

作者：

Lamarque, J. -F. ^{[1
]}

Bond, T. C. ^{[2
]}

Eyring, V. ^{[3
]}

Granier, C. ^{[4
,5
,6
]}

Heil, A. ^{[7
]}

Klimont, Z. ^{[8
]}

Lee, D. ^{[9
]}

Liousse, C. ^{[10
]}

Mieville, A. ^{[6
]}

Owen, B. ^{[9
]}

Schultz, M. G. ^{[7
]}

Shindell, D. ^{[11
]}

Smith, S. J. ^{[12
]}

Stehfest, E. ^{[13
]}

Van Aardenne, J. ^{[14
]}

Cooper, O. R. ^{[5
]}

Kainuma, M. ^{[15
]}

Mahowald, N. ^{[16
]}

McConnell, J. R. ^{[17
]}

Naik, V. ^{[18
]}

Riahi, K. ^{[8
]}

van Vuuren, D. P. ^{[13
]}

机构：

[1] Natl Ctr Atmospher Res, Boulder, CO 80307 USA

[2] Univ Illinois, Urbana, IL 61801 USA

[3] Deutsch Zentrum Luft & Raumfahrt DLR, Inst Phys Atmosphare, Oberpfaffenhoffen, Germany

[4] NOAA, Earth Syst Res Lab, Div Chem Sci, Boulder, CO USA

[5] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA

[6] Univ Paris 06, CNRS, UPMC, INSU,LATMOS IPSL,UMR 8190, Paris, France

[7] Forschungszentrum Julich, D-52425 Julich, Germany

[8] Int Inst Appl Syst Anal, A-2361 Laxenburg, Austria

[9] Manchester Metropolitan Univ, Manchester M15 6BH, Lancs, England

[10] Lab Aerol, Toulouse, France

[11] Natl Aeronaut & Space Agcy, Goddard Inst Space Studies, New York, NY USA

[12] Pacific NW Natl Lab, Joint Global Change Res Inst, College Pk, MD USA

[13] Netherlands Environm Assessment Agcy, Bilthoven, Netherlands

[14] Commiss European Communities, Joint Res Ctr, DG, I-21020 Ispra, Italy

[15] Natl Inst Environm Studies, Tsukuba, Ibaraki, Japan

[16] Cornell Univ, Ithaca, NY USA

[17] Univ Nevada, Desert Res Inst, Reno, NV 89506 USA

[18] NOAA, High Performance Technol Inc, Geophys Fluid Dynam Lab, Princeton, NJ USA

来源：

ATMOSPHERIC CHEMISTRY AND PHYSICS | 2010年 / 10卷 / 15期

基金：

美国国家科学基金会;

关键词：

CARBONACEOUS PARTICLES; TRACE GASES; FOSSIL-FUEL; CLIMATE; OZONE; PERIOD; SIMULATIONS; INVENTORY; SCENARIOS; DIOXIDE;

D O I：

10.5194/acp-10-7017-2010

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

We present and discuss a new dataset of gridded emissions covering the historical period (1850-2000) in decadal increments at a horizontal resolution of 0.5 degrees in latitude and longitude. The primary purpose of this inventory is to provide consistent gridded emissions of reactive gases and aerosols for use in chemistry model simulations needed by climate models for the Climate Model Intercomparison Program #5 (CMIP5) in support of the Intergovernmental Panel on Climate Change (IPCC) Fifth Assessment report (AR5). Our best estimate for the year 2000 inventory represents a combination of existing regional and global inventories to capture the best information available at this point; 40 regions and 12 sectors are used to combine the various sources. The historical reconstruction of each emitted compound, for each region and sector, is then forced to agree with our 2000 estimate, ensuring continuity between past and 2000 emissions. Simulations from two chemistry-climate models are used to test the ability of the emission dataset described here to capture long-term changes in atmospheric ozone, carbon monoxide and aerosol distributions. The simulated long-term change in the Northern mid-latitudes surface and mid-troposphere ozone is not quite as rapid as observed. However, stations outside this latitude band show much better agreement in both present-day and long-term trend. The model simulations indicate that the concentration of carbon monoxide is underestimated at the Mace Head station; however, the long-term trend over the limited observational period seems to be reasonably well captured. The simulated sulfate and black carbon deposition over Greenland is in very good agreement with the ice-core observations spanning the simulation period. Finally, aerosol optical depth and additional aerosol diagnostics are shown to be in good agreement with previously published estimates and observations.

引用

页码：7017 / 7039

页数：23

共 122 条

[1] Emission of trace gases and aerosols from biomass burning [J].