Structure, magnetic properties and magnetoelastic anisotropy in epitaxial Sr(Ti1-xCox)O3 films

被引：48

作者：

Bi, Lei ^{[1
]}

Kim, Hyun-Suk ^{[1
]}

Dionne, Gerald F. ^{[1
,2
]}

Ross, C. A. ^{[1
]}

机构：

[1] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA

[2] MIT, Lincoln Lab, Lexington, MA 02420 USA

来源：

NEW JOURNAL OF PHYSICS | 2010年 / 12卷

基金：

美国国家科学基金会;

关键词：

TRANSPORT-PROPERTIES; OXYGEN; FERROMAGNETISM; PHOTOEMISSION; STRESS; OXIDES; SRTIO3;

D O I：

10.1088/1367-2630/12/4/043044

中图分类号：

O4 [物理学];

学科分类号：

0702 ;

摘要：

We report the structure, magnetic properties and magnetoelastic anisotropy of epitaxial Sr(Ti1-xCox)O-3 films grown on LaAlO3 (001) and SrTiO3 (001) substrates by pulsed laser deposition. Room temperature ferromagnetism was observed in the Sr(Ti0.86Co0.14)O-3 and Sr(Ti0.77Co0.23)O-3 films. The formation of magnetic secondary phases such as Co-metal clusters in Sr(Ti0.77Co0.23)O-3 is excluded based on x-ray diffraction, cross-sectional TEM, x-ray photoelectron spectroscopy and x-ray-absorption near edge spectroscopy. A large magnetic anisotropy is observed in Sr(Ti0.77Co0.23)O-3 films. The net anisotropy is strongly influenced by growth conditions and the substrate and is attributed to magnetoelastic effects. The magnetoelastic anisotropy is related to the valence and spin states of the Co ions, which contribute to the ferromagnetic properties. Magneto-optical characterization yields a figure of merit (Faraday rotation/optical absorption) of 0.57 deg dB(-1) in the Sr(Ti0.77Co0.23)O-3 film at 1550 nm wavelength, making it potentially useful in integrated magneto-optical applications.

引用

页数：15

共 36 条

[1]

BALLHAUSEN CJ, 1962, INTRODUCTION LIGAND, pCH10

[2] Structural, magnetic, and magneto-optical properties of Co-doped CeO2-δ films [J].