Fundamental limits on third-order molecular susceptibilities

被引：143

作者：

Kuzyk, MG ^{[1
]}

机构：

[1] Washington State Univ, Dept Phys, Pullman, WA 99164 USA

来源：

OPTICS LETTERS | 2000年 / 25卷 / 16期

关键词：

D O I：

10.1364/OL.25.001183

中图分类号：

O43 [光学];

学科分类号：

070207 ; 0803 ;

摘要：

By the use of sum rules, the largest third-order molecular nonlinear-optical susceptibilities allowed by quantum mechanics are determined. The theoretical upper limit is found to depend only on the first excited-state transition energy and on the number of electrons, in agreement with experimental data. (C) 2000 Optical Society of America. OCIS codes: 190.0190, 160.0160, 160.4330.

引用

页码：1183 / 1185

页数：3

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