Magneto-resistance and superparamagnetism in magnetite films on MgO and MgAl2O4

被引:45
作者
Eerenstein, W [1 ]
Kalev, L [1 ]
Niesen, L [1 ]
Palstra, TTM [1 ]
Hibma, T [1 ]
机构
[1] Univ Groningen, Ctr Mat Sci, Dept Phys Chem, NL-9747 AG Groningen, Netherlands
关键词
magneto-resistance; spin polarization; superparamagnetism; magnetite; spinel;
D O I
10.1016/S0304-8853(02)01109-5
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The present study is a comparison of the resistive and magnetic properties of ultrathin epitaxial Fe3O4 films grown on MgO(001) and MgAl2O4(001). Such films on MgO are known to contain anti-phase boundaries, which cause magneto-resistance in these films, an increased resistivity with respect to the bulk and superparamagnetic behaviour for films below 5 nm thickness. Ultrathin films on MgAl2O4 show a very similar behaviour as the resistivity is also increased with respect to the bulk, but is still lower than the resistivity of films grown on MgO. This indicates a larger domain size in the films grown on MgAl2O4. This is supported by the observed magneto-resistance that is larger than for films grown on MgO. Mossbauer spectroscopy analysis of a 1.7 nm thick film on MgO indicates that all magnetic moments in the film are fluctuating, whereas for the film on MgAl2O4 a sextet with a parabolic background is observed. This shows that some domains are small enough for the moment to fluctuate while in larger ones, the moments are fixed; this also indicates that the domains in the film on MgAl2O4 are larger than in the film grown on MgO. (C) 2002 Elsevier Science B.V. All rights reserved.
引用
收藏
页码:73 / 76
页数:4
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