Dynamically induced frustration as a route to a quantum spin ice state in Tb2Ti2O7 via virtual crystal field excitations and quantum many-body effects

被引:227
作者
Molavian, Hamid R. [1 ]
Gingras, Michel J. P.
Canals, Benjamin
机构
[1] Univ Waterloo, Dept Phys & Astron, Waterloo, ON N2L 3G1, Canada
[2] Univ Canterbury, Dept Phys & Astron, Christchurch, New Zealand
[3] CNRS, Inst Neel, F-38042 Grenoble 9, France
[4] Univ Grenoble 1, F-38042 Grenoble 9, France
关键词
D O I
10.1103/PhysRevLett.98.157204
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The Tb2Ti2O7 pyrochlore magnetic material is attracting much attention for its spin liquid state, failing to develop long-range order down to 50 mK despite a Curie-Weiss temperature theta(CW) similar to -14 K. In this Letter we reinvestigate the theoretical description of this material by considering a quantum model of independent tetrahedra to describe its low-temperature properties. The naturally tuned proximity of this system near a Neel to spin ice phase boundary allows for a resurgence of quantum fluctuation effects that lead to an important renormalization of its effective low-energy spin Hamiltonian. As a result, Tb2Ti2O7 is argued to be a quantum spin ice. We put forward an experimental test of this proposal using neutron scattering on a single crystal.
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共 38 条
[1]   Quantum effects in a half-polarized pyrochlore antiferromagnet [J].
Bergman, DL ;
Shindou, R ;
Fiete, GA ;
Balents, L .
PHYSICAL REVIEW LETTERS, 2006, 96 (09)
[2]   Direct evidence for a dynamical ground state in the highly frustrated Tb2Sn2O7 pyrochlore [J].
Bert, F. ;
Mendels, P. ;
Olariu, A. ;
Blanchard, N. ;
Collin, G. ;
Amato, A. ;
Baines, C. ;
Hillier, A. D. .
PHYSICAL REVIEW LETTERS, 2006, 97 (11)
[3]   Magnetic frustration on a Kagome lattice in R3Ga5SiO14 langasites with R = Nd, Pr [J].
Bordet, P. ;
Gelard, I. ;
Marty, K. ;
Ibanez, A. ;
Robert, J. ;
Simonet, V. ;
Canals, B. ;
Ballou, R. ;
Lejay, P. .
JOURNAL OF PHYSICS-CONDENSED MATTER, 2006, 18 (22) :5147-5153
[4]   Spin ice state in frustrated magnetic pyrochlore materials [J].
Bramwell, ST ;
Gingras, MJP .
SCIENCE, 2001, 294 (5546) :1495-1501
[5]   Spin correlations in Ho2Ti2O7:: A dipolar spin ice system -: art. no. 047205 [J].
Bramwell, ST ;
Harris, MJ ;
den Hertog, BC ;
Gingras, MJP ;
Gardner, JS ;
McMorrow, DF ;
Wildes, AR ;
Cornelius, AL ;
Champion, JDM ;
Melko, RG ;
Fennell, T .
PHYSICAL REVIEW LETTERS, 2001, 87 (04) :47205-1
[6]   Ice: A strongly correlated proton system [J].
Castro Neto, A. H. ;
Pujol, P. ;
Fradkin, Eduardo .
PHYSICAL REVIEW B, 2006, 74 (02)
[7]  
CHIN A, CONDMAT0610544
[8]   Short-range magnetic interactions in the spin-ice compound HO2Ti2O7 -: art. no. 060406 [J].
Cornelius, AL ;
Gardner, JS .
PHYSICAL REVIEW B, 2001, 64 (06) :604061-604063
[9]   Quantum spin fluctuations in the dipolar Heisenberg-like rare earth pyrochlores [J].
Del Maestro, AG ;
Gingras, MJP .
JOURNAL OF PHYSICS-CONDENSED MATTER, 2004, 16 (20) :3339-3353
[10]   Dipolar interactions and origin of spin ice in Ising pyrochlore magnets [J].
den Hertog, BC ;
Gingras, MJP .
PHYSICAL REVIEW LETTERS, 2000, 84 (15) :3430-3433