Theory of sub-picosecond exciton motion in photosynthetic antenna systems

被引：3

作者：

May, V ^{[1
]}

Renger, T ^{[1
]}

机构：

[1] Humboldt Univ, Inst Phys, D-10117 Berlin, Germany

来源：

APPLIED PHYSICS B-LASERS AND OPTICS | 2000年 / 71卷 / 03期

关键词：

D O I：

10.1007/s003400000349

中图分类号：

O43 [光学];

学科分类号：

070207 ; 0803 ;

摘要：

Recent achievements in the theoretical description of exciton transfer in photosynthetic antennae are reviewed. Emphasis is put on the role of the protein matrix in the process of excitation energy dissipation. The computations are based on the standard Frenkel-exciton model including some necessary extensions. To carry out the simulations of experimental spectra the density-matrix theory is utilized. A numerical Monte Carlo treatment is applied to account for structural and energetic disorder. The approach is used to interpret various measurements on photosynthetic antenna systems. In particular, it is demonstrated how the exciton spectrum can be used as a probe for the protein spectral density.

引用

页码：451 / 456

页数：6

共 32 条

[1]

Agranovich V.M., 1982, Electronic Excitation Energy Transfer in Condensed Matter

[2]

Blum K., 2012, DENSITY MATRIX THEOR

[3] Third-order optical response of intermediate excitons with fractional nonlinear statistics [J].

Chernyak, V ;

Mukamel, S .

JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS, 1996, 13 (06) :1302-1307

[4] Four-wave mixing and luminescence of confined excitons in molecular aggregates and nanostructures. Many-body Green function approach [J].

Chernyak, V ;

Wang, NJ ;

Mukamel, S .

PHYSICS REPORTS-REVIEW SECTION OF PHYSICS LETTERS, 1995, 263 (4-6) :213-309

[5]

Davydov A. S., 1962, THEORY MOL EXCITONS

[6] CHLOROPHYLL ARRANGEMENT IN A BACTERIOCHLOROPHYLL PROTEIN FROM CHLOROBIUM-LIMICOLA [J].

FENNA, RE ;

MATTHEWS, BW .

NATURE, 1975, 258 (5536) :573-577

[7] Exciton dynamics in FMO bacteriochlorophyll protein at low temperatures [J].

Freiberg, A ;

Lin, S ;

Timpmann, K ;

Blankenship, RE .

JOURNAL OF PHYSICAL CHEMISTRY B, 1997, 101 (37) :7211-7220

[8] APPLICATION OF A MULTILEVEL REDFIELD THEORY TO ELECTRON-TRANSFER IN CONDENSED PHASES [J].

JEAN, JM ;

FRIESNER, RA ;

FLEMING, GR .

JOURNAL OF CHEMICAL PHYSICS, 1992, 96 (08) :5827-5842

[9]

Kasha M., 1976, SPECTROSCOPY EXCITED, P337, DOI DOI 10.1007/978-1-4684-2793-6_12

[10]

KENKRE VM, 1982, SPRINGER TRACTS MOD, V94

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