Coexistence of the critical slowing down and glassy freezing in relaxor ferroelectrics

被引:46
作者
Vugmeister, BE [1 ]
Rabitz, H [1 ]
机构
[1] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA
关键词
D O I
10.1103/PhysRevB.61.14448
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We have developed a dynamical model for the dielectric response in relaxor ferroelectrics that explicitly takes into account the coexistence of the critical slowing down and glassy freezing. The application of the model to the experiment in PbMg1/3Nb2/3O3 (PMN) allowed for the reconstruction of the nonequilibrium spin-glass state order parameter and its comparison with the results of recent NMR experiment [R. Blinc er al., Phys. Rev. Lett 83, 424 (1999)]. It is shown that the degree of the local freezing is rather small even at temperatures where the held-cooled permittivity exceeds the frequency-dependent permittivity by an order of magnitude. This observation indicates the significant role of the critical slowing down (accompanying the glass freezing) in the system dynamics. Also, the theory predicts an important interrelationship between the frequency-dependent permittivity and the zero-field-cooled permittivity, which proved to be consistent with the experiment in PMN.
引用
收藏
页码:14448 / 14453
页数:6
相关论文
共 22 条
[1]   SPIN-GLASSES - EXPERIMENTAL FACTS, THEORETICAL CONCEPTS, AND OPEN QUESTIONS [J].
BINDER, K ;
YOUNG, AP .
REVIEWS OF MODERN PHYSICS, 1986, 58 (04) :801-976
[2]   Local polarization distribution and Edwards-Anderson order parameter of relaxor ferroelectrics [J].
Blinc, R ;
Dolinsek, J ;
Gregorovic, A ;
Zalar, B ;
Filipic, C ;
Kutnjak, Z ;
Levstik, A ;
Pirc, R .
PHYSICAL REVIEW LETTERS, 1999, 83 (02) :424-427
[3]  
Blinc R., 1974, SOFT MODES FERROELEC
[4]   FERROELECTRICS WITH A GLASSY POLARIZATION PHASE [J].
BURNS, G ;
DACOL, FH .
FERROELECTRICS, 1990, 104 :25-35
[5]   VOGEL-FULCHER SCALING OF THE SUSCEPTIBILITY IN A MIXED-CRYSTAL PROTON GLASS [J].
COURTENS, E .
PHYSICAL REVIEW LETTERS, 1984, 52 (01) :69-72
[6]  
CROSS LE, 1987, FERROELECTRICS, V76, P241, DOI 10.2109/jcersj.99.829
[7]   A STRUCTURAL MODEL FOR THE RELAXOR PBMG1/3NB2/3O3 AT 5-K [J].
DEMATHAN, N ;
HUSSON, E ;
CALVARIN, G ;
GAVARRI, JR ;
HEWAT, AW ;
MORELL, A .
JOURNAL OF PHYSICS-CONDENSED MATTER, 1991, 3 (42) :8159-8171
[8]   Nature of atomic ordering and mechanism of relaxor ferroelectric phenomena it PMN [J].
Egami, T ;
Dmowski, W ;
Teslic, S ;
Davies, PK ;
Chen, IW ;
Chen, H .
FERROELECTRICS, 1998, 206 (1-4) :231-244
[9]   Evidence for domain-type dynamics in the ergodic phase of the PbMg1/3Nb2/3O3 relaxor ferroelectric [J].
Glazounov, AE ;
Tagantsev, AK ;
Bell, AJ .
PHYSICAL REVIEW B, 1996, 53 (17) :11281-11284
[10]  
Glinchuk MD, 1997, J APPL PHYS, V81, P3561, DOI 10.1063/1.364993