Magnetic instabilities in Fe3C cementite particles observed with FeK-edge X-ray circular dichroism under pressure -: art. no. 075502

被引:65
作者
Duman, E
Acet, M [1 ]
Wassermann, EF
Itié, JP
Baudelet, F
Mathon, O
Pascarelli, S
机构
[1] Univ Duisburg Gesamthsch, D-47048 Duisburg, Germany
[2] Univ Paris 06, CNRS, UMR 7602, F-75252 Paris 05, France
[3] Syncrotron Soleil Orme Merisiers, F-91192 Gif Sur Yvette, France
[4] European Synchrotron Radiat Facil, F-38043 Grenoble, France
关键词
D O I
10.1103/PhysRevLett.94.075502
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The ferromagnetic interstitial iron compound Fe3C (cementite) is expected to have Invar properties, whereby a high-moment to low-moment transition should occur when the atomic volume is reduced below a critical value. We, therefore, examine the pressure dependence of the Fe K-edge x-ray magnetic circular dichroism in Fe3C at ambient temperature and pressures up to 20 GPa. We find clear evidence for a high-moment to low-moment transition around 10 GPa.
引用
收藏
页数:4
相关论文
共 26 条
[1]   MAGNETISM AT HIGH-PRESSURE IN FCC FE-BASED ALLOYS [J].
ABDELMEGUID, MM ;
MICKLITZ, H .
PHYSICA B, 1989, 161 (1-3) :17-21
[2]   Relevance of magnetic instabilities to the properties of interstitial solid solutions and compounds of Fe [J].
Acet, M ;
Gehrmann, B ;
Wassermann, EF ;
Bach, H ;
Pepperhoff, W .
JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS, 2001, 232 (03) :221-230
[3]   Relativistic calculations of spin-dependent x-ray-absorption spectra [J].
Ankudinov, AL ;
Rehr, JJ .
PHYSICAL REVIEW B, 1997, 56 (04) :R1712-R1715
[4]   Multiple-scattering theory of x-ray magnetic circular dichroism: Implementation and results for the iron K edge [J].
Brouder, C ;
Alouani, M ;
Bennemann, KH .
PHYSICAL REVIEW B, 1996, 54 (10) :7334-7349
[5]   Abrupt discontinuity of the bulk modulus pressure dependence in Fe64Ni36 -: art. no. 157204 [J].
Decremps, F ;
Nataf, L .
PHYSICAL REVIEW LETTERS, 2004, 92 (15) :157204-1
[6]   Large spontaneous magnetostrictive softening below the Curie temperature of Fe3C Invar particles [J].
Duman, E ;
Acet, M ;
Hülser, T ;
Wassermann, EF ;
Rellinghaus, B ;
Itié, JP ;
Munsch, P .
JOURNAL OF APPLIED PHYSICS, 2004, 96 (10) :5668-5672
[7]   THEORY OF CIRCULARLY POLARIZED X-RAY ABSORPTION BY FERROMAGNETIC FE [J].
EBERT, H ;
STRANGE, P ;
GYORFFY, BL .
JOURNAL OF APPLIED PHYSICS, 1988, 63 (08) :3055-3057
[8]   1ST-PRINCIPLES CALCULATIONS OF THE INSTABILITY LEADING TO THE INVAR EFFECT [J].
ENTEL, P ;
HOFFMANN, E ;
MOHN, P ;
SCHWARZ, K ;
MORUZZI, VL .
PHYSICAL REVIEW B, 1993, 47 (14) :8706-8720
[9]   Spin- and orbital-polarized multiple-scattering theory of magneto-x-ray effects in Fe, Co, and Ni [J].
Guo, GY .
PHYSICAL REVIEW B, 1997, 55 (17) :11619-11628
[10]   ELECTRONIC-STRUCTURE, X-RAY PHOTOEMISSION SPECTRA, AND TRANSPORT-PROPERTIES OF FE3C (CEMENTITE) [J].
HAGLUND, J ;
GRIMVALL, G ;
JARLBORG, T .
PHYSICAL REVIEW B, 1991, 44 (07) :2914-2919