Three pulse echo peak shift measurements on the B820 subunit of LH1 of Rhodospirillum rubrum

被引:74
作者
Yu, JY
Nagasawa, Y
van Grondelle, R
Fleming, GR
机构
[1] Univ Chicago, Dept Chem, Chicago, IL 60637 USA
[2] Univ Chicago, James Franck Inst, Chicago, IL 60637 USA
[3] Vrije Univ Amsterdam, Fac Phys & Astron, Dept Biophys, NL-1081 HV Amsterdam, Netherlands
基金
美国国家科学基金会;
关键词
D O I
10.1016/S0009-2614(97)01135-4
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Three pulse photon echo peak shift measurements (3PEPS) of the detergent isolated B820 subunit of the light harvesting complex of Rhodospirillum rubrum are presented and compared with 3PEPS data for the LH1 complex of Rhodobacter sphaeroides. The comparison suggests that the 90 fs component of LH1 3PEPS is indeed the energy transfer component. The striking similarity between 3PEPS of LH1 and B820 subunit also suggests that excitation is delocalized over only a dimer unit. (C) 1997 Elsevier Science B.V.
引用
收藏
页码:404 / 410
页数:7
相关论文
共 35 条
[1]   EXCITATION TRANSFER IN THE CORE LIGHT-HARVESTING COMPLEX (LH-1) OF RHODOBACTER-SPHAEROIDES - AN ULTRAFAST FLUORESCENCE DEPOLARIZATION AND ANNIHILATION STUDY [J].
BRADFORTH, SE ;
JIMENEZ, R ;
VANMOURIK, F ;
VANGRONDELLE, R ;
FLEMING, GR .
JOURNAL OF PHYSICAL CHEMISTRY, 1995, 99 (43) :16179-16191
[2]   ISOLATION AND CHARACTERIZATION OF A STRUCTURAL SUBUNIT FROM THE CORE LIGHT-HARVESTING COMPLEX OF RHODOBACTER-SPHAEROIDES 2.4.1 AND PUC705-BA [J].
CHANG, MC ;
MEYER, L ;
LOACH, PA .
PHOTOCHEMISTRY AND PHOTOBIOLOGY, 1990, 52 (04) :873-881
[3]  
CHO M, 1997, COMMUNICATION
[4]   PHOTON-ECHO MEASUREMENTS IN LIQUIDS - NUMERICAL-CALCULATIONS WITH MODEL SYSTEMS [J].
CHO, MH ;
FLEMING, GR .
JOURNAL OF CHEMICAL PHYSICS, 1993, 98 (04) :2848-2859
[5]   The integrated photon echo and solvation dynamics [J].
Cho, MH ;
Yu, JY ;
Joo, TH ;
Nagasawa, Y ;
Passino, SA ;
Fleming, GR .
JOURNAL OF PHYSICAL CHEMISTRY, 1996, 100 (29) :11944-11953
[6]   X-RAY STRUCTURE-ANALYSIS OF A MEMBRANE-PROTEIN COMPLEX - ELECTRON-DENSITY MAP AT 3A RESOLUTION AND A MODEL OF THE CHROMOPHORES OF THE PHOTOSYNTHETIC REACTION CENTER FROM RHODOPSEUDOMONAS-VIRIDIS [J].
DEISENHOFER, J ;
EPP, O ;
MIKI, K ;
HUBER, R ;
MICHEL, H .
JOURNAL OF MOLECULAR BIOLOGY, 1984, 180 (02) :385-398
[7]   GENETICALLY MODIFIED PHOTOSYNTHETIC ANTENNA COMPLEXES WITH BLUESHIFTED ABSORBENCY BANDS [J].
FOWLER, GJS ;
VISSCHERS, RW ;
GRIEF, GG ;
VANGRONDELLE, R ;
HUNTER, CN .
NATURE, 1992, 355 (6363) :848-850
[8]   LINEAR VIBRONIC COUPLING IN A GENERAL 2 LEVEL SYSTEM [J].
FRIESNER, RA ;
SILBEY, R .
JOURNAL OF CHEMICAL PHYSICS, 1981, 75 (08) :3925-3936
[9]   REVERSIBLE DISSOCIATION OF THE B873 LIGHT-HARVESTING COMPLEX FROM RHODOSPIRILLUM-RUBRUM G9+ [J].
GHOSH, R ;
HAUSER, H ;
BACHOFEN, R .
BIOCHEMISTRY, 1988, 27 (03) :1004-1014
[10]   FEMTOSECOND ENERGY-TRANSFER WITHIN THE LH2 PERIPHERAL ANTENNA OF THE PHOTOSYNTHETIC PURPLE BACTERIA RHODOBACTER-SPHAEROIDES AND RHODOPSEUDOMONAS-PALUSTRIS LL [J].
HESS, S ;
FELDCHTEIN, F ;
BABIN, A ;
NURGALEEV, I ;
PULLERITS, T ;
SERGEEV, A ;
SUNDSTROM, V .
CHEMICAL PHYSICS LETTERS, 1993, 216 (3-6) :247-257