Alternating layer and island growth of Pb on Si by spontaneous quantum phase separation

被引:83
作者
Hong, HW
Wei, CM
Chou, MY
Wu, Z
Basile, L
Chen, H
Holt, M
Chiang, TC
机构
[1] Univ Illinois, Frederick Seitz Mat Res Lab, Urbana, IL 61801 USA
[2] Acad Sinica, Inst Phys, Taipei 11529, Taiwan
[3] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA
[4] Univ Illinois, Dept Mat Sci & Engn, Urbana, IL 61801 USA
[5] Univ Illinois, Dept Phys, Urbana, IL 61801 USA
[6] City Univ Hong Kong, Dept Phys & Mat Sci, Kowloon, Hong Kong, Peoples R China
关键词
D O I
10.1103/PhysRevLett.90.076104
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Real-time in situ x-ray studies of continuous Pb deposition on Si(111)-(7x7) at 180 K reveal an unusual growth behavior. A wetting layer forms first to cover the entire surface. Then islands of a fairly uniform height of about five monolayers form on top of the wetting layer and grow to fill the surface. The growth then switches to a layer-by-layer mode upon further deposition. This behavior of alternating layer and island growth can be attributed to spontaneous quantum phase separation based on a first-principles calculation of the system energy.
引用
收藏
页数:4
相关论文
共 17 条
[1]   Electron fringes on a quantum wedge [J].
Altfeder, IB ;
Matveev, KA ;
Chen, DM .
PHYSICAL REVIEW LETTERS, 1997, 78 (14) :2815-2818
[2]   Extracting convergent surface formation energies from slab calculations [J].
Boettger, JC ;
Smith, JR ;
Birkenheuer, U ;
Rosch, N ;
Trickey, SB ;
Sabin, JR ;
Apell, SP .
JOURNAL OF PHYSICS-CONDENSED MATTER, 1998, 10 (04) :893-894
[3]   Uniform, self-organized, seven-step height Pb/Si(111)-(7X7) islands at low temperatures [J].
Budde, K ;
Abram, E ;
Yeh, V ;
Tringides, MC .
PHYSICAL REVIEW B, 2000, 61 (16) :10602-10605
[4]   Photoemission studies of quantum well states in thin films [J].
Chiang, TC .
SURFACE SCIENCE REPORTS, 2000, 39 (7-8) :181-235
[5]  
CRACKNELL AP, 1984, METALS PHONON EL 13C, V3, P275
[6]   Novel growth of Ag islands on Si(III): Plateaus with a singular height [J].
Gavioli, L ;
Kimberlin, KR ;
Tringides, MC ;
Wendelken, JF ;
Zhang, ZY .
PHYSICAL REVIEW LETTERS, 1999, 82 (01) :129-132
[7]   Uniform island height selection in the low temperature growth of Pb/Si(111)-(7 x 7) [J].
Hupalo, M ;
Kremmer, S ;
Yeh, V ;
Berbil-Bautista, L ;
Abram, E ;
Tringides, MC .
SURFACE SCIENCE, 2001, 493 (1-3) :526-538
[8]   ELECTRONIC SHELL STRUCTURE AND ABUNDANCES OF SODIUM CLUSTERS [J].
KNIGHT, WD ;
CLEMENGER, K ;
DEHEER, WA ;
SAUNDERS, WA ;
CHOU, MY ;
COHEN, ML .
PHYSICAL REVIEW LETTERS, 1984, 52 (24) :2141-2143
[9]   Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set [J].
Kresse, G ;
Furthmuller, J .
PHYSICAL REVIEW B, 1996, 54 (16) :11169-11186
[10]   Quantum electronic stability of atomically uniform films [J].
Luh, DA ;
Miller, T ;
Paggel, JJ ;
Chou, MY ;
Chiang, TC .
SCIENCE, 2001, 292 (5519) :1131-1133