Electroabsorption in single-crystal film of a second-order optical material

被引:7
作者
Swamy, RK [1 ]
Kutty, SP [1 ]
Titus, J [1 ]
Khatavkar, S [1 ]
Thakur, M [1 ]
机构
[1] Auburn Univ, Photon Mat Res Lab, Auburn, AL 36849 USA
基金
美国国家科学基金会;
关键词
D O I
10.1063/1.1811772
中图分类号
O59 [应用物理学];
学科分类号
摘要
In this letter, we report results of electroabsorption and resonant electro-optic measurements in single-crystal film of 4(')-dimethylamino-N-methyl-4-stilbazolium tosylate (DAST). The electroabsorption measurement was made by recording the changes in transmission through the film as an ac field was applied along the dipole axis. The electro-optic measurement was made using the field-induced birefringence method. The measurements were made in the absorptive domain, at 633 and 488 nm. The modulation (DeltaT/T) due to electroabsorption decreased as the angle between the incident polarization and the dipole axis was increased. The observed electroabsorption is due to the imaginary part of the electro-optic coefficient. The real part of the electro-optic coefficient (r(11)) as measured at 633 nm is 770 pm/V. The imaginary parts of the electro-optic coefficients at 633 and 488 nm are 104 and 259 pm/V, respectively. (C) 2004 American Institute of Physics.
引用
收藏
页码:4025 / 4027
页数:3
相关论文
共 9 条
[1]   Electroabsorption of a new urethane-substituted polydiacetylene PDA-5BCMU-4A in a film [J].
Jia, WY ;
Misawa, K ;
Matsuda, H ;
Okada, S ;
Nakanishi, H ;
Kobayashi, T .
CHEMICAL PHYSICS LETTERS, 1996, 255 (4-6) :385-392
[2]   ORGANIC SALTS WITH LARGE 2ND-ORDER OPTICAL NONLINEARITIES [J].
MARDER, SR ;
PERRY, JW ;
YAKYMYSHYN, CP .
CHEMISTRY OF MATERIALS, 1994, 6 (08) :1137-1147
[3]   ELECTRIC-FIELD DEPENDENCE OF LINEAR OPTICAL-PROPERTIES IN QUANTUM-WELL STRUCTURES - WAVE-GUIDE ELECTROABSORPTION AND SUM-RULES [J].
MILLER, DAB ;
WEINER, JS ;
CHEMLA, DS .
IEEE JOURNAL OF QUANTUM ELECTRONICS, 1986, 22 (09) :1816-1830
[4]   Electro-optic properties of the organic salt 4-N,N-dimethylamino-4'-N'-methyl-stilbazolium tosylate [J].
Pan, F ;
Knopfle, G ;
Bosshard, C ;
Follonier, S ;
Spreiter, R ;
Wong, MS ;
Gunter, P .
APPLIED PHYSICS LETTERS, 1996, 69 (01) :13-15
[5]   Single-pass thin-film electro-optic modulator based on an organic molecular salt [J].
Thakur, M ;
Xu, JJ ;
Bhowmik, A ;
Zhou, LG .
APPLIED PHYSICS LETTERS, 1999, 74 (05) :635-637
[6]   GROWTH OF LARGE-AREA THIN-FILM SINGLE-CRYSTALS OF POLY(DIACETYLENES) [J].
THAKUR, M ;
MEYLER, S .
MACROMOLECULES, 1985, 18 (11) :2341-2344
[7]   Electro-optic modulation at 1.5 GHz using single-crystal film of an organic molecular salt [J].
Thakur, M ;
Mishra, A ;
Titus, J ;
Ahyi, AC .
APPLIED PHYSICS LETTERS, 2002, 81 (20) :3738-3740
[8]  
THAKUR M, 1989, SYNTHETIC MET, V28, P595
[9]   QUADRATIC ELECTROOPTIC EFFECT DUE TO THE QUANTUM-CONFINED STARK-EFFECT IN QUANTUM-WELLS [J].
WEINER, JS ;
MILLER, DAB ;
CHEMLA, DS .
APPLIED PHYSICS LETTERS, 1987, 50 (13) :842-844