Electron-Phonon Coupling in CdSe Nanocrystals

被引:110
作者
Kelley, Anne Myers [1 ]
机构
[1] Univ Calif Merced, Sch Nat Sci, Merced, CA 95343 USA
来源
JOURNAL OF PHYSICAL CHEMISTRY LETTERS | 2010年 / 1卷 / 09期
关键词
RESONANCE RAMAN-SPECTROSCOPY; SIZE DEPENDENCE; QUANTUM DOTS; SEMICONDUCTOR MICROCRYSTALLITES; EXCITON; SCATTERING; PHOTOLUMINESCENCE; STATE; LIMIT;
D O I
10.1021/jz100123b
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The coupling between nuclear vibrations and electronic excitations (electron-phonon coupling) in semiconductor nanocrystals influences many photophysical process in these materials. While electron-phonon coupling in CdSe nanocrystals has been studied both experimentally and theoretically for more than 20 years, there remains little agreement about its magnitude and size dependence. This perspective summarizes key litreature results suggests reasons for their disagreement, and proposes approaches to better determine this important quantity.
引用
收藏
页码:1296 / 1300
页数:5
相关论文
共 31 条
[1]   ELECTRON-VIBRATION COUPLING IN SEMICONDUCTOR CLUSTERS STUDIED BY RESONANCE RAMAN-SPECTROSCOPY [J].
ALIVISATOS, AP ;
HARRIS, TD ;
CARROLL, PJ ;
STEIGERWALD, ML ;
BRUS, LE .
JOURNAL OF CHEMICAL PHYSICS, 1989, 90 (07) :3463-3468
[2]   Effect of ZnS shell thickness on the phonon spectra in CdSe quantum dots [J].
Baranov, AV ;
Rakovich, YP ;
Donegan, JF ;
Perova, TS ;
Moore, RA ;
Talapin, DV ;
Rogach, AL ;
Masumoto, Y ;
Nabiev, I .
PHYSICAL REVIEW B, 2003, 68 (16)
[3]   Direct observation of confined acoustic phonons in the photoluminescence spectra of a single CdSe-CdS-ZnS core-shell-shell nanocrystal [J].
Chilla, Gerwin ;
Kipp, Tobias ;
Menke, Torben ;
Heitmann, Detlef ;
Nikolic, Marija ;
Froemsdorf, Andreas ;
Kornowski, Andreas ;
Foerster, Stephan ;
Weller, Horst .
PHYSICAL REVIEW LETTERS, 2008, 100 (05)
[4]   TIME-RESOLVED VIBRATIONAL SPECTROSCOPY IN THE IMPULSIVE LIMIT [J].
DHAR, L ;
ROGERS, JA ;
NELSON, KA .
CHEMICAL REVIEWS, 1994, 94 (01) :157-193
[5]   The influence of shell parameters on phonons in core-shell nanoparticles: a resonant Raman study [J].
Dzhagan, V. M. ;
Valakh, M. Ya ;
Raevska, O. E. ;
Stroyuk, O. L. ;
Kuchmiy, S. Ya ;
Zahn, D. R. T. .
NANOTECHNOLOGY, 2009, 20 (36)
[6]   Size effects on Raman spectra of small CdSe nanoparticles in polymer films [J].
Dzhagan, V. M. ;
Valakh, M. Ya ;
Raevskaya, A. E. ;
Stroyuk, A. L. ;
Kuchmiy, S. Ya ;
Zahn, D. R. T. .
NANOTECHNOLOGY, 2008, 19 (30)
[7]  
Empedocles SA, 1999, ADV MATER, V11, P1243, DOI 10.1002/(SICI)1521-4095(199910)11:15<1243::AID-ADMA1243>3.0.CO
[8]  
2-2
[9]   Acoustic phonon contributions to the emission spectrum of single CdSe nanocrystals [J].
Fernee, Mark J. ;
Littleton, Brad N. ;
Cooper, Steven ;
Rubinsztein-Dunlop, Halina ;
Gomez, Daniel E. ;
Mulvaney, Paul .
JOURNAL OF PHYSICAL CHEMISTRY C, 2008, 112 (06) :1878-1884
[10]   SIMPLE ASPECTS OF RAMAN-SCATTERING [J].
HELLER, EJ ;
SUNDBERG, RL ;
TANNOR, D .
JOURNAL OF PHYSICAL CHEMISTRY, 1982, 86 (10) :1822-1833