Global climate response to anthropogenic aerosol indirect effects: Present day and year 2100

被引:25
作者
Chen, Wei-Ting [1 ]
Nenes, Athanasios [2 ,3 ]
Liao, Hong [4 ]
Adams, Peter J. [5 ,6 ]
Li, Jui-Lin F.
Seinfeld, John H. [1 ,7 ]
机构
[1] CALTECH, Dept Environm Sci & Engn, Pasadena, CA 91125 USA
[2] Georgia Inst Technol, Sch Earth & Atmospher Sci, Atlanta, GA 30332 USA
[3] Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA
[4] Chinese Acad Sci, LAPC, Inst Atmospher Phys, Beijing 100029, Peoples R China
[5] Carnegie Mellon Univ, Dept Civil & Environm Engn, Pittsburgh, PA 15213 USA
[6] Carnegie Mellon Univ, Dept Engn & Publ Policy, Pittsburgh, PA 15213 USA
[7] CALTECH, Dept Chem Engn, Pasadena, CA 91125 USA
基金
美国国家航空航天局; 中国国家自然科学基金;
关键词
GENERAL-CIRCULATION MODEL; DROPLET GROWTH-KINETICS; ORGANIC AEROSOL; CLOUD PARAMETERIZATION; CCN ACTIVITY; SULFATE; CONDENSATION; SIMULATIONS; SENSITIVITY; ACTIVATION;
D O I
10.1029/2008JD011619
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
Aerosol indirect effects (AIE) are a principal source of uncertainty in future climate predictions. The present study investigates the equilibrium response of the climate system to present-day and future AIE using the general circulation model (GCM), Goddard Institute for Space Studies (GISS) III. A diagnostic formulation correlating cloud droplet number concentration (N-c) with concentrations of aerosol soluble ions is developed as a basis for the calculation. Explicit dependence on Nc is introduced in the treatments of liquid-phase stratiform clouds in GISS III. The model is able to reproduce the general patterns of present-day cloud frequency, droplet size, and radiative balance observed by CloudSat, Moderate Resolution Imaging Spectroradiometer, and Earth Radiation Budget Experiment. For perturbations of N-c from preindustrial to present day, a net AIE forcing of -1.67 W m(-2) is estimated, with a global mean surface cooling of 1.12 K, precipitation reduction of 3.36%, a southward shift of the Intertropical Convergence Zone, and a hydrological sensitivity of + 3.00% K-1. For estimated perturbations of N-c from present day to year 2100, a net AIE forcing of -0.58 W m(-2), a surface cooling of 0.47 K, and a decrease in precipitation of 1.7% are predicted. Sensitivity calculations show that the assumption of a background minimum N-c value has more significant effects on AIE forcing in the future than on that in present day. When AIE-related processes are included in the GCM, a decrease in stratiform precipitation is predicted over future greenhouse gas (GHG)-induced warming scenario, as opposed to the predicted increase when only GHG and aerosol direct effects are considered.
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页数:23
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