Removal of SO2 and NO from flue gas by wet scrubbing using an aqueous NaClO2 solution

被引:164
作者
Chien, TW [1 ]
Chu, H [1 ]
机构
[1] Natl Cheng Kung Univ, Dept Environm Engn, Tainan 70101, Taiwan
关键词
wet scrubber; absorption; sodium chlorite; nitric oxide; flue gas; wet scrubbing;
D O I
10.1016/S0304-3894(00)00274-0
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
This study used a NaClO2/NaOH solution as the additive/absorbent to determine the extent of NOx removal in a wet scrubbing system. A combined SOx/NOx removal system was also tested. The experiments were performed in a bench-scale spraying sieve tray wet scrubber in a continuous mode. The operating variables included NO and SO2 concentrations, L/G ratio, molar ratio, and initial pH. The results of the individual DeNO(x) experiments show that the maximum DeNO(x) efficiencies ranged from 3.1 to 12.6%. The results of the combined DeSO(x)/DeNO(x) experiments show that the maximum DeNO(x) and DeSO(x) efficiencies ranged from 36.6 to 71.9% and from 89.4 to 100.0%, respectively. The major parameters affecting NO, removal efficiencies are the L/G ratio and the dosage of additive. The major parameter influencing DeSO(x) efficiencies is the L/G ratio. (C) 2000 Elsevier Science B.V. All rights reserved.
引用
收藏
页码:43 / 57
页数:15
相关论文
共 17 条
[1]  
[Anonymous], 1990, GAS SEP PURIF, DOI DOI 10.1016/j.jhazmat.2008.08.056
[2]  
Brogren C, 1998, CHEM ENG TECHNOL, V21, P61, DOI 10.1002/(SICI)1521-4125(199801)21:1<61::AID-CEAT61>3.0.CO
[3]  
2-0
[4]  
CHAN KF, 1991, THESIS U WINDSOR ONT
[5]   LBL PHOSNOX PROCESS FOR COMBINED REMOVAL OF SO2 AND NOX FROM FLUE-GAS [J].
CHANG, SG ;
LEE, GC .
ENVIRONMENTAL PROGRESS, 1992, 11 (01) :66-73
[6]   Absorption of NO by NaClO2 solution:: Performance characteristics [J].
Hsu, HW ;
Lee, CJ ;
Chou, KS .
CHEMICAL ENGINEERING COMMUNICATIONS, 1998, 170 :67-81
[7]  
JOSHI JB, 1988, CHEM ENG COMMUN, V33, P1
[8]   REMOVAL OF NITROGEN-OXIDES WITH AQUEOUS-SOLUTIONS OF INORGANIC AND ORGANIC-REAGENTS [J].
KOBAYASHI, H ;
TAKEZAWA, N ;
NIKI, T .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1977, 11 (02) :190-192
[9]  
NOVOSELOV SS, 1986, THERM ENG+, V33, P496
[10]   ABSORPTION OF LEAN NOX IN AQUEOUS-SOLUTIONS OF NACLO2 AND NAOH [J].
SADA, E ;
KUMAZAWA, H ;
KUDO, I ;
KONDO, T .
INDUSTRIAL & ENGINEERING CHEMISTRY PROCESS DESIGN AND DEVELOPMENT, 1979, 18 (02) :275-278