An assessment of the impact of climate change on air quality at two UK sites

被引:23
作者
Athanassiadou, Maria [1 ]
Baker, Jonathan [1 ]
Carruthers, David [2 ]
Collins, William [1 ]
Girnary, Sofia [2 ]
Hassell, David [3 ]
Hort, Matthew [1 ]
Johnson, Colin [1 ]
Johnson, Kate [2 ]
Jones, Richard [3 ]
Thomson, David [1 ]
Trought, Nicki [2 ]
Witham, Claire [1 ]
机构
[1] Met Off, Hadley Ctr, Exeter EX1 3PB, Devon, England
[2] Cambridge Environm Res Consultants Ltd, Cambridge CB2 1SJ, England
[3] Univ Reading, Met Off, Hadley Ctr, Reading Unit, Reading RG6 6BB, Berks, England
关键词
Climate change; Air quality; Urban pollution; Dispersion modelling; Ozone; Nitrogen Oxides; PM10; SURFACE OZONE; DISPERSION; MODEL; ADMS; EUROPE; SYSTEM;
D O I
10.1016/j.atmosenv.2010.02.024
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Possible effects of climate change on air quality are studied for two urban sites in the UK, London and Glasgow. Hourly meteorological data were obtained from climate simulations for two periods representing the current climate and a plausible late 21st century climate. Of the meteorological quantities relevant to air quality, significant changes were found in temperature, specific humidity, wind speed, wind direction, cloud cover, solar radiation, surface sensible heat flux and precipitation. Using these data, dispersion estimates were made for a variety of single sources and some significant changes in environmental impact were found in the future climate. In addition, estimates for future background concentrations of NOx, NO2, ozone and PM10 upwind of London and Glasgow were made using the meteorological data in a statistical model. These showed falls in NOx and increases in ozone for London, while a fall in NO2 was the largest percentage change for Glasgow. Other changes were small. With these background estimates, annual-average concentrations of NOx. NO2, ozone and PM10 were estimated within the two urban areas. For London, results averaged over a number of sites showed a fall in NOx and a rise in ozone, but only small changes in NO2 and PM10. For Glasgow, the changes in all four chemical species were small. Large-scale background ozone values from a global chemical transport model are also presented. These show a decrease in background ozone due to climate change. To assess the net impact of both large scale and local processes will require models which treat all relevant scales. Crown Copyright (C) 2010 Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码:1877 / 1886
页数:10
相关论文
共 29 条
[1]  
*AIR QUAL EXP GROU, 2007, AIR QUAL CLIM CHANG
[2]  
[Anonymous], 2002, CLIMATE CHANGE SCENA
[3]   On the robustness of changes in extreme precipitation over Europe from two high resolution climate change simulations [J].
Buonomo, E. ;
Jones, R. ;
Huntingford, C. ;
Hannaford, J. .
QUARTERLY JOURNAL OF THE ROYAL METEOROLOGICAL SOCIETY, 2007, 133 (622) :65-81
[4]   Removal of chlorofluorocarbons by increased mass exchange between the stratosphere and troposphere in a changing climate [J].
Butchart, N ;
Scaife, AA .
NATURE, 2001, 410 (6830) :799-802
[5]  
CARRUTHERS D, 2006, LOCAL IMPACT CLIMATE
[6]   UK-ADMS - A NEW APPROACH TO MODELING DISPERSION IN THE EARTHS ATMOSPHERIC BOUNDARY-LAYER [J].
CARRUTHERS, DJ ;
HOLROY, DRJ ;
HUNT, JCR ;
WENG, WS ;
ROBINS, AG ;
APSLEY, DD ;
THOMSON, DJ ;
SMITH, FB .
JOURNAL OF WIND ENGINEERING AND INDUSTRIAL AERODYNAMICS, 1994, 52 (1-3) :139-153
[7]  
*CERC, 2005, ADMS 3 TECHN SPEC
[8]  
*CERC, 2003, RUR PRED US GUID VER
[9]   Effect of stratosphere-troposphere exchange on the future tropospheric ozone trend [J].
Collins, WJ ;
Derwent, RG ;
Garnier, B ;
Johnson, CE ;
Sanderson, MG ;
Stevenson, DS .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2003, 108 (D12)
[10]   Tropospheric ozone in a global-scale three-dimensional Lagrangian model and its response to NOX emission controls [J].
Collins, WJ ;
Stevenson, DS ;
Johnson, CE ;
Derwent, RG .
JOURNAL OF ATMOSPHERIC CHEMISTRY, 1997, 26 (03) :223-274