Optimal quantum control with multi-polarization fields

被引：7

作者：

Wu, R ^{[1
]}

Sola, IR ^{[1
]}

Rabitz, H ^{[1
]}

机构：

[1] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA

来源：

CHEMICAL PHYSICS LETTERS | 2004年 / 400卷 / 4-6期

基金：

美国国家科学基金会;

关键词：

D O I：

10.1016/j.cplett.2004.10.151

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

The dynamical advantages for employing up to three independently shaped polarization fields are explored in the optimal control of quantum systems. The analysis compares multi-polarization optimal control with what may be achieved using linearly polarized (1-D) control. Simulations on model systems show how multi-polarization (2-D, 3-D) optimally shaped pulses can overcome symmetry forbidden transitions and improve control quality by better accessibility to the target state. (C) 2004 Elsevier B.V. All rights reserved.

引用

页码：469 / 475

页数：7

共 30 条

[1] Generation and characterization of polarization-shaped femtosecond laser pulses
Brixner, T
Krampert, G
Niklaus, P
Gerber, G
[J]. APPLIED PHYSICS B-LASERS AND OPTICS, 2002, 74 (Suppl 1): : S133 - S144
[2] Femtosecond polarization pulse shaping
Brixner, T
Gerber, G
[J]. OPTICS LETTERS, 2001, 26 (08) : 557 - 559
[3] Brumer P., 2001, Phys. Rev. A, V65, DOI DOI 10.1103/PHYSREVA.65.015401
[4] Laser coherent control of molecular chiral states via entanglement of the rotational and torsional degrees of freedom
Bychkov, SS
Grishanin, BA
Zadkov, VN
Takahashi, H
[J]. JOURNAL OF RAMAN SPECTROSCOPY, 2002, 33 (11-12) : 962 - 973
[5] Laser synthesis of chiral molecules in isotropic racemic media
Bychkov, SS
Grishanin, BA
Zadkov, VN
[J]. JOURNAL OF EXPERIMENTAL AND THEORETICAL PHYSICS, 2001, 93 (01) : 24 - 32
[6] ON THE PREPARATION AND MEASUREMENT OF SUPERPOSITIONS OF CHIRAL AMPLITUDES
CINA, JA
HARRIS, RA
[J]. JOURNAL OF CHEMICAL PHYSICS, 1994, 100 (04) : 2531 - 2536
[7] Unity occupation of sites in a 3D optical lattice
DePue, MT
McCormick, C
Winoto, SL
Oliver, S
Weiss, DS
[J]. PHYSICAL REVIEW LETTERS, 1999, 82 (11) : 2262 - 2265
[8] Experiments with a 3D double optical lattice
Ellmann, H
Jersblad, J
Kastberg, A
[J]. PHYSICAL REVIEW LETTERS, 2003, 90 (05) : 4
[9] Enantiomeric purification of nonpolarized racemic mixtures using coherent light
Frishman, E
Shapiro, M
Gerbasi, D
Brumer, P
[J]. JOURNAL OF CHEMICAL PHYSICS, 2003, 119 (14) : 7237 - 7246
[10] Fujimura Y, 2000, ANGEW CHEM INT EDIT, V39, P4586, DOI 10.1002/1521-3773(20001215)39:24<4586::AID-ANIE4586>3.0.CO

← 1 2 3 →