Orbital-order-induced metal-insulator transition in La1-xCaxMnO3

被引:93
作者
Van Aken, BB [1 ]
Jurchescu, OD
Meetsma, A
Tomioka, Y
Tokura, Y
Palstra, TTM
机构
[1] Univ Groningen, Ctr Mat Sci, Solid State Chem Lab, Nijenborgh 4, NL-9747 AG Groningen, Netherlands
[2] AIST, CERC, Tsukuba, Ibaraki 3058562, Japan
[3] AIST, JRCAT, Tsukuba, Ibaraki 3050046, Japan
[4] Univ Tokyo, Dept Appl Phys, Bunkyo Ku, Tokyo 1138656, Japan
关键词
D O I
10.1103/PhysRevLett.90.066403
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We present evidence that the insulator-to-metal transition in La1-xCaxMnO3 near x similar to 0.2 is driven by the suppression of coherent Jahn-Teller distortions, originating from d-type orbital ordering. The orbital-ordered state is characterized by large long-range Q2 distortions below TO'-O*. Above TO'-O* we find evidence for coexistence between an orbital-ordered and an orbital-disordered state. This behavior is discussed in terms of electronic phase separation in an orbital-ordered insulating and an orbital-disordered metallic state.
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页数:4
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