Long-term variation of black carbon and PM2.5 in Beijing, China with respect to meteorological conditions and governmental measures

被引:102
作者
Chen, Yuan [1 ]
Schleicher, Nina [1 ]
Fricker, Mathieu [2 ]
Cen, Kuang [3 ]
Liu, Xiu-li [3 ]
Kaminski, Uwe [2 ]
Yu, Yang [3 ]
Wu, Xue-fang [3 ]
Norra, Stefan [1 ,4 ,5 ]
机构
[1] Karlsruhe Inst Technol, Inst Appl Geosci, Working Grp Environm Mineral & Environm Syst Anal, D-76131 Karlsruhe, Germany
[2] German Meteorol Serv, Dept Air Qual, Res Ctr Human Biometeorol, D-79104 Freiburg, Germany
[3] China Univ Geosci, Sch Earth Sci & Resources, Beijing 100083, Peoples R China
[4] Karlsruhe Inst Technol, Inst Geog & Geoecol, D-76131 Karlsruhe, Germany
[5] Tech Univ Bergakad Freiberg, Inst Mineral, Brennhausgasse 14, D-09596 Freiberg, Germany
关键词
Urban aerosol; PM2.5; Black carbon; Temporal distribution; Megacity; PARTICULATE ELEMENTAL CARBON; SUMMER GAMES 2008; MITIGATION MEASURES; ORGANIC-CARBON; MASS CONCENTRATIONS; EMISSIONS; AEROSOLS; PARTICLES; ASSOCIATIONS; ATMOSPHERE;
D O I
10.1016/j.envpol.2016.01.008
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Black carbon (BC) and PM2.5 were studied for nine years from 2005 to 2013 in the Beijing urban area. The overall weekly average mass concentrations of BC and PM2.5 were 4.3 and 66.8 mu g/m(3). PM2.5 annual means of the nine years are around 2 times of the standard (GB3095-2012) in China, and are 5-7 times higher than the WHO standard. The Beijing Olympic Games in 2008 was a milestone to mitigate aerosol pollution. Temporal distribution of BC shows a distinct declining trend, and annual mean mass concentrations of PM2.5 after 2008 were lower than those before 2008 but increased from 2011 to 2013. Wind rose plots show that high BC concentrations are usually associated with low wind speed of northeastern or southwestern winds, generally causing poor visibility. Governmental mitigation measures such as traffic restriction despite increased motor vehicle numbers and gasoline consumption and industry relocation with declining consumption of coal and coke were successful in reducing BC emissions. Annual mean of BC was reduced by 38% in 2013 compared to 2005. However, BC contamination in Beijing is still severe when compared to other urban areas around the world. (C) 2016 Elsevier Ltd. All rights reserved.
引用
收藏
页码:269 / 278
页数:10
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