Radiative absorption, fluorescence, and scattering of a classical dipole near a lossless interface: a unified description

被引:118
作者
Mertz, J [1 ]
机构
[1] Ecole Super Phys & Chim Ind Ville Paris, INSERM, EPI00 02, Physiol Lab, F-75231 Paris, France
关键词
D O I
10.1364/JOSAB.17.001906
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
A simple input-output formalism based on the Lorentz reciprocity theorem is presented for the study of a classical radiating dipole near a lossless interface. The problems of dipole absorption, fluorescence, and scattering are considered in a unified description, and the effects of the interface (a simple dielectric here) are shown to be broadly twofold. First, the channeling of radiation into and out of the dipole is modified. Second, the intrinsic dipole polarizability is found to be modified, leading to an effective absorption (or scattering) cross section that depends on the states of both the dipole and the driving field. These results are particularly applicable to studies involving evanescent-wave microscopy. (C) 2000 Optical Society of America [S0740-3224(00)01211-X].
引用
收藏
页码:1906 / 1913
页数:8
相关论文
共 26 条
[1]  
Axelrod D, 1991, TOPICS FLUORESCENCE, V3, P289
[2]  
Born M., 1986, PRINCIPLES OPTICS
[3]   ABSORPTION AND EMISSION OF EVANESCENT PHOTONS [J].
CARNIGLIA, CK ;
MANDEL, L ;
DREXHAGE, KH .
JOURNAL OF THE OPTICAL SOCIETY OF AMERICA, 1972, 62 (04) :479-+
[4]  
Chance R. R., 1978, ADV CHEM PHYS, V37, P1, DOI DOI 10.1002/9780470142561.CH1
[5]   LIFETIME OF AN EMITTING MOLECULE NEAR A PARTIALLY REFLECTING SURFACE [J].
CHANCE, RR ;
PROCK, A ;
SILBEY, R .
JOURNAL OF CHEMICAL PHYSICS, 1974, 60 (07) :2744-2748
[6]   FREQUENCY-SHIFTS OF AN ELECTRIC-DIPOLE TRANSITION NEAR A PARTIALLY REFLECTING SURFACE [J].
CHANCE, RR ;
PROCK, A ;
SILBEY, R .
PHYSICAL REVIEW A, 1975, 12 (04) :1448-1452
[7]   SURFACE-ENHANCED 2ND-HARMONIC GENERATION AND RAMAN-SCATTERING [J].
CHEN, CK ;
HEINZ, TF ;
RICARD, D ;
SHEN, YR .
PHYSICAL REVIEW B, 1983, 27 (04) :1965-1979
[8]   Internal dynamics of multilevel atoms near a vacuum-dielectric interface [J].
Courtois, JY ;
Courty, JM ;
Mertz, JC .
PHYSICAL REVIEW A, 1996, 53 (03) :1862-1878
[9]   Simultaneous imaging of individual molecules aligned both parallel and perpendicular to the optic axis [J].
Dickson, RM ;
Norris, DJ ;
Moerner, WE .
PHYSICAL REVIEW LETTERS, 1998, 81 (24) :5322-5325
[10]   IMAGING OF SINGLE FLUORESCENT MOLECULES AND INDIVIDUAL ATP TURNOVERS BY SINGLE MYOSIN MOLECULES IN AQUEOUS-SOLUTION [J].
FUNATSU, T ;
HARADA, Y ;
TOKUNAGA, M ;
SAITO, K ;
YANAGIDA, T .
NATURE, 1995, 374 (6522) :555-559