Photoionization of NaI: inward-outward asymmetry in the wave packet detection

被引:32
作者
Gregoire, G [1 ]
Mons, M
Dimicoli, I
Piuzzi, F
Charron, E
Dedonder-Lardeux, C
Jouvet, C
Martrenchard, S
Solgadi, D
Suzor-Weiner, A
机构
[1] CEA Saclay, SPAM, DRECAM, F-91911 Gif Sur Yvette, France
[2] Universite Paris Sud, CNRS, Photophys Mol Lab, F-91405 Orsay, France
[3] CEA Saclay, Lab Rech Correspondant, LRC DSM 9702, F-91911 Gif Sur Yvette, France
[4] Chim Phys Lab, F-75231 Paris 05, France
关键词
D O I
10.1007/s100530050079
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
The nuclear wave packet in the A state of NaI has been monitored in a pump-probe femtosecond experiment using a resonant two-photon ionization detection scheme. A strong asymmetry depending on the direction of propagation of the wave packet is observed in the Na+ ion signal. This phenomenon; well reproduced by a full quantum wave packet calculation, has been assigned to the combination of two effects: i) the motion of the wave packet in the intermediate state of the two-photon probe process, ii) the R-dependence of the photoionization efficiency of this intermediate state.
引用
收藏
页码:187 / 192
页数:6
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