Magnetic tunneling told to ignorants by two ignorants

被引:29
作者
Villain, J
Fort, A
机构
[1] CNRS, Ctr Rech Tres Basses Temp, F-38042 Grenoble 9, France
[2] Commissariat Energie Atom, Dept Rech Fondamentale Mat Condensee, F-38054 Grenoble 9, France
[3] Univ Florence, Dipartimento Fis, Ist Nazl Fis Mat, Unita Firenze, I-50125 Florence, Italy
关键词
D O I
10.1007/s100510070161
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
Magnetic tunneling of a large spin subject to the Hamiltonian H = -DSz2 + BSx2 - g mu(B)H . S is investigated by elementary methods for weak fields H. In zero field (H = 0) the tunnel frequency in the ground state is found to be equal to Ds[1 + (2D/B) + 2 root(1 + D/B)D/B](-s) multiplied by a quantity whose variation with s is slower than exponential. This result coincides with that of path integral methods [16]. For the values of the longitudinal field which allow tunneling, the tunnel frequency w(T) is shown to vanish when H-y = 0 for certain "diabolic" values of g mu(B)H(x)/root B(D + B), in qualitative agreement with experiments by Wernsdorfer and Sessoli. The particular case H-z = 0 was already obtained by Garg by means of path integrals. The diabolic values of g mu(B)H(x)/root B(D + B) are in agreement with numerical results but, as already noticed by Wernsdorfer and Sessoli, they disagree with the experimental ones. This may be an effect of higher order anisotropy terms, which is briefly addressed in the conclusion.
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页码:69 / 83
页数:15
相关论文
共 32 条
[1]   QUANTUM OSCILLATIONS IN SMALL MAGNETIC PARTICLES [J].
BOGACHEK, EN ;
KRIVE, IV .
PHYSICAL REVIEW B, 1992, 46 (22) :14559-14562
[2]   DISCRETE SEMICLASSICAL METHODS IN THE THEORY OF RYDBERG ATOMS IN EXTERNAL FIELDS [J].
BRAUN, PA .
REVIEWS OF MODERN PHYSICS, 1993, 65 (01) :115-161
[3]   The molecular approach to nanoscale magnetism [J].
Caneschi, A ;
Gatteschi, D ;
Sangregorio, C ;
Sessoli, R ;
Sorace, L ;
Cornia, A ;
Novak, MA ;
Paulsen, C ;
Wernsdorfer, W .
JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS, 1999, 200 (1-3) :182-201
[4]   Macroscopic quantum coherence in molecular magnets [J].
Chiolero, A ;
Loss, D .
PHYSICAL REVIEW LETTERS, 1998, 80 (01) :169-172
[5]   QUANTUM INTERFERENCE IS SMALL MAGNETIC PARTICLES [J].
CHUDNOVSKY, EM ;
DIVINCENZO, DP .
PHYSICAL REVIEW B, 1993, 48 (14) :10548-10551
[6]   QUANTUM TUNNELING OF MAGNETIZATION IN SMALL FERROMAGNETIC PARTICLES [J].
CHUDNOVSKY, EM ;
GUNTHER, L .
PHYSICAL REVIEW LETTERS, 1988, 60 (08) :661-664
[7]   Dipolar interaction and incoherent quantum tunneling: a Monte Carlo study of magnetic relaxation [J].
Cuccoli, A ;
Fort, A ;
Rettori, A ;
Adam, E ;
Villain, J .
EUROPEAN PHYSICAL JOURNAL B, 1999, 12 (01) :39-46
[8]  
DINGLE RB, 1967, APPL SCI RES, V18, P238
[9]  
EINSTEIN A, 1967, EVOLUTION PHYSICS
[10]   SPIN TUNNELING IN THE SEMICLASSICAL LIMIT [J].
ENZ, M ;
SCHILLING, R .
JOURNAL OF PHYSICS C-SOLID STATE PHYSICS, 1986, 19 (11) :1765-1770