Aerosol optical, chemical and physical properties at Gosan, Korea during Asian dust and pollution episodes in 2001

被引:83
作者
Kim, SW
Yoon, SC
Jefferson, A
Ogren, JA
Dutton, EG
Won, JG
Ghim, YS
Lee, IB
Han, JS
机构
[1] NOAA, Climate Monitoring & Diagnost Lab, Boulder, CO 80305 USA
[2] Seoul Natl Univ, Sch Earth & Environm Sci, Seoul, South Korea
[3] Korea Inst Sci & Technol, Air Resource Res Ctr, Seoul 130650, South Korea
[4] Natl Inst Environm Res, Div Atmospher Chem, Inchon, South Korea
关键词
Asian dust and pollution; light scattering; light absorption; aerosol radiative forcing; Gosan;
D O I
10.1016/j.atmosenv.2004.09.056
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
In order to understand the influence of dust and anthropogenic pollution aerosols on regional climate in East Asia. we analyzed the aerosol optical, chemical and physical properties for two cases with high aerosol loading and assessed the radiative forcing of these cases. The 1st case study is a heavy dust episode (DE) in April (during ACE-Asia) 2001 and the 2nd case is a regional-scale pollution event in November 2001. The Angstrom exponent (Angstrom) for DE was. VIS from sunphotometer measurements. The mean single scattering albedo (550 nm) at the surface reported during the pollution episode (PE, 0.88) was lower than that of DE (0.91). The concentrations of organic (OC) and elemental carbon (EC) measured during the PE were about 90% and 30% higher than DE. The aerosol mass scattering efficency (alpha(s)) of PE is a factor of about 2 higher than that of the DE. The difference in the mass absorption efficiency (z(a)) of EC during DE and PE is small and within the measurement uncertainty. The diurnally averaged aerosol radiative forcing efficiency (DeltaDFE, W m(-2) tau(-1)) during DE is similar to results of other studies at Gosan. (C) 2004 Elsevier Ltd. All rights reserved.
引用
收藏
页码:39 / 50
页数:12
相关论文
共 30 条
[1]   Variability of aerosol optical properties derived from in situ aircraft measurements during ACE-Asia [J].
Anderson, TL ;
Masonis, SJ ;
Covert, DS ;
Ahlquist, NC ;
Howell, SG ;
Clarke, AD ;
McNaughton, CS .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2003, 108 (D23)
[2]  
ANDREWS E, 2001, SUMM REPORT, V26, P60
[3]  
[Anonymous], 2001, Climate Change 2001:Impacts, Adaptation and Vulnerability
[4]   Aerosol radiative, physical, and chemical properties in Beijing during June 1999 [J].
Bergin, MH ;
Cass, GR ;
Xu, J ;
Fang, C ;
Zeng, LM ;
Yu, T ;
Salmon, LG ;
Kiang, CS ;
Tang, XY ;
Zhang, YH ;
Chameides, WL .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2001, 106 (D16) :17969-17980
[5]   Surface aerosol radiative forcing at Gosan during the ACE-Asia campaign [J].
Bush, BC ;
Valero, FPJ .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2003, 108 (D23)
[6]   Mixtures of pollution, dust, sea salt, and volcanic aerosol during ACE-Asia: Radiative properties as a function of relative humidity [J].
Carrico, CM ;
Kus, P ;
Rood, MJ ;
Quinn, PK ;
Bates, TS .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2003, 108 (D23)
[7]  
김영성, 2003, [Journal of Korean Society for Atmospheric Environment , 한국대기환경학회지], V19, P469
[8]  
CLARK A, 2004, J GEOPHYSICAL RES, V109
[9]   A model for the radiative forcing during ACE-Asia derived from CIRPAS Twin Otter and R/V Ronald H. Brown data and comparison with observations [J].
Conant, WC ;
Seinfeld, JH ;
Wang, J ;
Carmichael, GR ;
Tang, YH ;
Uno, I ;
Flatau, PJ ;
Markowicz, KM ;
Quinn, PK .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2003, 108 (D23)
[10]  
Delene DJ, 2002, J ATMOS SCI, V59, P1135, DOI 10.1175/1520-0469(2002)059<1135:VOAOPA>2.0.CO