Characterization of Cu-CeO2 direct hydrocarbon anodes in a solid oxide fuel cell with lanthanum gallate electrolyte

被引:51
作者
An, S
Lu, C
Worrell, WL
Gorte, RJ
Vohs, JM
机构
[1] Univ Penn, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA
[2] Univ Penn, Dept Chem & Biomol Engn, Philadelphia, PA 19104 USA
关键词
intermediate temperature; solid oxide fuel cells; doped lanthanum gallate; Cu-CeO2-LSGM anodes; impedance spectroscopy;
D O I
10.1016/j.ssi.2004.09.029
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
La0.8Sr0.2Ga0.8Mg0.2O3-delta (LSGM)-electrolyte-supported solid oxide fuel cells (SOFCs)with Cu-CeO2-LSGM anodes were fabricated, and their performance, while operating on H-2 and C4H10, was characterized. The cells demonstrated the ability to directly operate on both hydrogen and butane fuels between 600 and 700 degreesC. At 700 degreesC, a cell with a 440-mum thick electrolyte had maximum power densities of 220 and 115 mW/cm(2) for H-2 and C4H10 fuels, respectively. Impedance study indicates that the Cu-CeO2-LSGM anodes limit cell performance. (C) 2004 Published by Elsevier B.V.
引用
收藏
页码:135 / 138
页数:4
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