Spatiotemporal control of nanooptical excitations

被引：117

作者：

Aeschlimann, Martin ^{[2
,3
]}

Bauer, Michael ^{[4
]}

Bayer, Daniela ^{[2
,3
]}

Brixner, Tobias ^{[5
]}

Cunovic, Stefan ^{[1
]}

Dimler, Frank ^{[5
]}

Fischer, Alexander ^{[2
,3
]}

Pfeiffer, Walter ^{[1
]}

Rohmer, Martin ^{[2
,3
]}

Schneider, Christian ^{[2
,3
]}

Steeb, Felix ^{[2
,3
]}

Strueber, Christian ^{[1
]}

Voronine, Dmitri V. ^{[5
]}

机构：

[1] Univ Bielefeld, Fak Phys, D-33615 Bielefeld, Germany

[2] Tech Univ Kaiserslautern, Fachbereich Phys, D-67663 Kaiserslautern, Germany

[3] Tech Univ Kaiserslautern, Res Ctr OPTIMAS, D-67663 Kaiserslautern, Germany

[4] Univ Kiel, Inst Expt & Angew Phys, D-24118 Kiel, Germany

[5] Univ Wurzburg, Inst Phys & Theoret Chem, D-97074 Wurzburg, Germany

来源：

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA | 2010年 / 107卷 / 12期

关键词：

coherent control; nanophotonics; plasmonics; ultrafast spectroscopy;

D O I：

10.1073/pnas.0913556107

中图分类号：

O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];

学科分类号：

07 ; 0710 ; 09 ;

摘要：

The most general investigation and exploitation of light-induced processes require simultaneous control over spatial and temporal properties of the electromagnetic field on a femtosecond time and nanometer length scale. Based on the combination of polarization pulse shaping and time-resolved two-photon photoemission electron microscopy, we demonstrate such control over nanoscale spatial and ultrafast temporal degrees of freedom of an electromagnetic excitation in the vicinity of a nanostructure. The time-resolved cross-correlation measurement of the local photoemission yield reveals the switching of the nanolocalized optical near-field distribution with a lateral resolution well below the diffraction limit and a temporal resolution on the femtosecond time scale. In addition, successful adaptive spatiotemporal control demonstrates the flexibility of the method. This flexible simultaneous control of temporal and spatial properties of nanophotonic excitations opens new possibilities to tailor and optimize the light-matter interaction in spectroscopic methods as well as in nanophotonic applications.

引用

页码：5329 / 5333

页数：5

共 18 条

[1] Adaptive subwavelength control of nano-optical fields [J].

Aeschlimann, Martin ;

Bauer, Michael ;

Bayer, Daniela ;

Brixner, Tobias ;

Garcia de Abajo, F. Javier ;

Pfeiffer, Walter ;

Rohmer, Martin ;

Spindler, Christian ;

Steeb, Felix .

NATURE, 2007, 446 (7133) :301-304

[2] Ultrafast adaptive optical near-field control [J].

Brixner, T ;

de Abajo, FJG ;

Schneider, J ;

Spindler, C ;

Pfeiffer, W .

PHYSICAL REVIEW B, 2006, 73 (12)

[3] Nanoscopic ultrafast space-time-resolved spectroscopy [J].

Brixner, T ;

de Abajo, FJG ;

Schneider, J ;

Pfeiffer, W .

PHYSICAL REVIEW LETTERS, 2005, 95 (09)

[4] Generation and characterization of polarization-shaped femtosecond laser pulses [J].

Brixner, T ;

Krampert, G ;

Niklaus, P ;

Gerber, G .

APPLIED PHYSICS B-LASERS AND OPTICS, 2002, 74 (Suppl 1) :S133-S144

[5] Femtosecond polarization pulse shaping [J].

Brixner, T ;

Gerber, G .

OPTICS LETTERS, 2001, 26 (08) :557-559

[6]

BRUMER PW, 2003, PRINCIPLES QUANTUM C, P117

[7] Toward full spatiotemporal control on the nanoscale [J].

Durach, Maxim ;

Rusina, Anastasia ;

Stockman, Mark I. .

NANO LETTERS, 2007, 7 (10) :3145-3149

[8] High-harmonic generation by resonant plasmon field enhancement [J].

Kim, Seungchul ;

Jin, Jonghan ;

Kim, Young-Jin ;

Park, In-Yong ;

Kim, Yunseok ;

Kim, Seung-Woo .

NATURE, 2008, 453 (7196) :757-760

[9] Femtosecond imaging of surface plasmon dynamics in a nanostructured silver film [J].

Kubo, A ;

Onda, K ;

Petek, H ;

Sun, ZJ ;

Jung, YS ;

Kim, HK .

NANO LETTERS, 2005, 5 (06) :1123-1127

[10]

NOVOSEL L, 2006, P C TEL INF MIPRO 20, P134

← 1 2 →