Creating and detecting shaped Rydberg wave packets

被引:41
作者
Krause, JL
Schafer, KJ
Ben-Nun, M
Wilson, KR
机构
[1] Univ Florida, Quantum Theory Project, Gainesville, FL 32611 USA
[2] Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA
[3] Univ Calif San Diego, Dept Chem & Biochem, La Jolla, CA 92093 USA
关键词
D O I
10.1103/PhysRevLett.79.4978
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Inherently quantum mechanical, transient nanostructures with dynamics on a picosecond time scale can be produced by controlling the quantum dynamics of Rydberg electrons. Ultrashort, tailored light pulses are used to build structures in position and/or momentum space from the wave function of an electron. The optimal laser pulses required to make these structures can be computed and synthesized in the laboratory. As an example, we present a structure consisting of five peaks which acts as a time-dependent grating and can be detected via ultrafast extreme ultraviolet diffraction.
引用
收藏
页码:4978 / 4981
页数:4
相关论文
共 27 条
[1]  
Alber G., 1991, Physics Reports, V199, P231, DOI 10.1016/0370-1573(91)90058-T
[2]   Generation of 18-fs, multiterawatt pulses by regenerative pulse shaping and chirped-pulse amplification [J].
Barty, CPJ ;
Guo, T ;
LeBlanc, C ;
Raksi, F ;
RosePetruck, C ;
Squier, J ;
Wilson, KR ;
Yakovlev, VV ;
Yamakawa, K .
OPTICS LETTERS, 1996, 21 (09) :668-670
[3]   Direct imaging of excited electronic states using diffraction techniques: Theoretical considerations [J].
BenNun, M ;
Martinez, TJ ;
Weber, PM ;
Wilson, KR .
CHEMICAL PHYSICS LETTERS, 1996, 262 (3-4) :405-414
[4]  
BRONER I, 1994, J OPT SOC AM B, V11, P2457
[5]   LASER CONTROL OF MOLECULAR PROCESSES [J].
BRUMER, P ;
SHAPIRO, M .
ANNUAL REVIEW OF PHYSICAL CHEMISTRY, 1992, 43 :257-282
[6]   SYNTHESIS OF CRAFTED OPTICAL PULSES BY TIME DOMAIN MODULATION IN A FIBER-GRATING COMPRESSOR [J].
HANER, M ;
WARREN, WS .
APPLIED PHYSICS LETTERS, 1988, 52 (18) :1458-1461
[7]   RAMSEY INTERFERENCE IN STRONGLY DRIVEN RYDBERG SYSTEMS [J].
JONES, RR ;
RAMAN, CS ;
SCHUMACHER, DW ;
BUCKSBAUM, PH .
PHYSICAL REVIEW LETTERS, 1993, 71 (16) :2575-2578
[8]   IONIZATION OF RYDBERG ATOMS BY SUBPICOSECOND HALF-CYCLE ELECTROMAGNETIC PULSES [J].
JONES, RR ;
YOU, D ;
BUCKSBAUM, PH .
PHYSICAL REVIEW LETTERS, 1993, 70 (09) :1236-1239
[9]   New states of hydrogen in a circularly polarized electromagnetic field [J].
Kalinski, M ;
Eberly, JH .
PHYSICAL REVIEW LETTERS, 1996, 77 (12) :2420-2423
[10]   CONTROLLING THE FUTURE OF MATTER [J].
KOHLER, B ;
KRAUSE, JL ;
RAKSI, F ;
WILSON, KR ;
YAKOVLEV, VV ;
WHITNELL, RM ;
YAN, YJ .
ACCOUNTS OF CHEMICAL RESEARCH, 1995, 28 (03) :133-140