Thermal fluctuations of freely suspended smectic-A films from mesoscopic to molecular length scales

被引:31
作者
Mol, EAL [1 ]
Wong, GCL [1 ]
Petit, JM [1 ]
Rieutord, F [1 ]
deJeu, WH [1 ]
机构
[1] UNIV GRENOBLE 1, CEA,CNRS,UMR 585, DEPT RECH FONDEMANTALE MATIERE CONDENSEE, F-38054 GRENOBLE, FRANCE
关键词
D O I
10.1103/PhysRevLett.79.3439
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The thermal fluctuations of freely suspended smectic-A films have been studied with diffuse x-ray scattering. Using a (2 + 2) scattering geometry at a synchrotron source the spectral dependence of the displacement-displacement correlation function has been determined from mesoscopic to molecular dimensions. At long in-plane length scales the fluctuations of the smectic layers were found to be conformal; i.e., all layers of the film fluctuated in unison. At decreasing length scales conformality was progressively lost, starting between the top and bottom layers of the film.
引用
收藏
页码:3439 / 3442
页数:4
相关论文
共 29 条
[1]   CRITICAL-BEHAVIOR OF THE LAYER COMPRESSIONAL ELASTIC CONSTANT-B AT THE SMECTIC-A NEMATIC PHASE-TRANSITION [J].
BENZEKRI, M ;
MARCEROU, JP ;
NGUYEN, HT ;
ROUILLON, JC .
PHYSICAL REVIEW B, 1990, 41 (13) :9032-9037
[2]  
Chaikin P.M., 2007, PRINCIPLES CONDENSED
[3]   Grazing incidence surface scattering of X-rays [J].
Daillant, J ;
Quinn, K ;
Gourier, C ;
Rieutord, F .
JOURNAL OF THE CHEMICAL SOCIETY-FARADAY TRANSACTIONS, 1996, 92 (04) :505-513
[4]   ANALOGY BETWEEN SUPERCONDUCTORS AND SMECTICS-A [J].
DEGENNES, PG .
SOLID STATE COMMUNICATIONS, 1972, 10 (09) :753-&
[5]  
DEGENNES PG, 1993, PHYSICS LIQUID CRYST
[6]   ELASTIC-CONSTANTS OF NEMATIC LIQUID-CRYSTALLINE TERMINALLY SUBSTITUTED AZOXYBENZENES [J].
DEJEU, WH ;
CLAASSEN, WAP .
JOURNAL OF CHEMICAL PHYSICS, 1977, 67 (08) :3705-3712
[7]   STEP-BY-STEP THINNING OF FREESTANDING FILMS ABOVE THE SMECTIC-A-NEMATIC PHASE-TRANSITION [J].
DEMIKHOV, EI ;
DOLGANOV, VK ;
MELETOV, KP .
PHYSICAL REVIEW E, 1995, 52 (02) :R1285-R1287
[8]   ANGLE CALCULATIONS FOR A 2+2 SURFACE X-RAY DIFFRACTOMETER [J].
EVANSLUTTERODT, KW ;
TANG, MT .
JOURNAL OF APPLIED CRYSTALLOGRAPHY, 1995, 28 :318-326
[9]   ABSOLUTE MEASUREMENT OF THE CRITICAL-BEHAVIOR OF THE SMECTIC ELASTIC-CONSTANT OF BILAYER AND MONOLAYER SMECTIC-A LIQUID-CRYSTALS ON APPROACHING THE TRANSITION TO THE NEMATIC PHASE [J].
FISCH, MR ;
PERSHAN, PS ;
SORENSEN, LB .
PHYSICAL REVIEW A, 1984, 29 (05) :2741-2750
[10]   BEND AND SPLAY ELASTIC-CONSTANTS OF DIHEPTYLAZOXYBENZENE [J].
GARG, S ;
CRANDALL, KA ;
KHAN, AA .
PHYSICAL REVIEW E, 1993, 48 (02) :1123-1130