Ultraviolet photoelectron spectroscopy of Si-4 to Si-1000

被引：63

作者：

Astruc Hoffmann M. ^{[1
]}

Wrigge G. ^{[1
]}

Issendorff B.V. ^{[1
]}

Müller J. ^{[1
]}

Ganteför G. ^{[2
]}

Haberland H. ^{[1
]}

机构：

[1] Fakultät für Physik, Universität Freiburg, 79104 Freiburg

[2] Fachbereich Physik, Universität Konstanz

来源：

The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics | 2001年 / 16卷 / 1期

关键词：

PACS. 36.40.Mr Spectroscopy and geometrical structure of clusters – 33.60.Cv Ultraviolet and vacuum ultraviolet photoelectron spectra – 71.24.+q Electronic structure of clusters and nanoparticles;

D O I：

10.1007/s100530170048

中图分类号：

学科分类号：

摘要：

Using a new experimental setup we have measured UV (hv = 6.4 eV) photoelectron spectra of cold silicon cluster anions Si-n in a very broad size range. For sizes up to n = 46 the spectra exhibit rich structures. For larger sizes only smooth spectra have been obtained. No trace of a bandgap has been found even for clusters with more than 1000 atoms.

引用

页码：9 / 11

页数：2

共 8 条

[1] Pavesi L., Dal Negro L., Mazzoleni C., Franzo G., Priolo F., Nature, 408, (2000)
[2] Binggeli N., Chelikowsky J.R., Phys. Rev. Lett., 75, (1995)
[3] Mitas L., Grossmann J.C., Stich I., Tobik J., Phys. Rev. Lett., 84, (2000)
[4] Muller J., Liu B., Shvartsburg A., Ogut S., Chelikowsky J.R., Siu K.W.M., Ho K.-M., Gantefor G., Phys. Rev. Lett., 85, (2000)
[5] Hudgins R.R., Imai M., Jarrold M.F., Dugourd Ph., J. Chem. Phys., 111, (1999)
[6] Haberland H., Mall M., Moseler M., Qiang Y., Reiners Th., Thurner Y., J. Vac. Sci. Technol. A, 12, (1994)
[7] Cheshnovsky O., Yang S.H., Pettiette C.L., Craycraft M.J., Liu Y., Smalley R.E., Chem. Phys. Lett., 138, (1987)
[8] Maus M., Gantefor G., Eberhardt W., Appl. Phys. A, 70, (2000)

← 1 →