Effect of Cu doping at the Mn site on the transport aaand magnetic behaviors of La2/3Ca1/3MnO3

被引:18
作者
S.L. Yuan
Z.Y. Li
X.Y. Zeng
G.Q. Zhang
F. Tu
G. Peng
J. Liu
Y. Jiang
Y.P. Yang
C.Q. Tang
机构
[1] Huazhong University of Science and Technology,Department of Physics
来源
The European Physical Journal B - Condensed Matter and Complex Systems | 2001年 / 20卷 / 2期
关键词
75.30.Vn Colossal magnetoresistance; 75.30.Kz Magnetic phase boundaries (including magnetic transitions, metamagnetism, etc.); 75.25.+z Spin arrangements in magnetically ordered materials (including neutron and spin-polarized electron studies, synchrotron-source X-ray scattering, etc.);
D O I
10.1007/BF01315688
中图分类号
学科分类号
摘要
We show that the replacement of Mn with Cu, without any structure change, strongly affects the transport and magnetic behaviors in La2/3Ca1/3 Mn1-xCuxO 3 - δ (x?0.3). Doping largely shifts the insulator-metal transition towards the low-temperature regime and causes substantial enhancements in both resistance and magnetoresistance near the transition for doping range of x? 15%, and further doping to x≥ 20% shows insulating behavior. For 15% doping, the sample shows large magnetoresistances (∼104%) over the whole low temperature range. Magnetization measurement at helium temperature reveals that samples for x? 10% and ≥ 20% basically show ferromagnetic (FM) and antiferromagnetic (AF) behaviors, respectively, while the 15% Cu doped sample undergoes a metamagnetic transition from AF state to FM state on increasing field. We argue that doping introduces the AF insulating phase into the system, causing unusual transport and magnetic behaviors.
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页码:177 / 181
页数:4
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