OBSERVATION OF ELECTRONIC-STRUCTURE AT THE METAL ELECTROLYTE AND METAL VACUUM INTERFACE BY 2ND-HARMONIC GENERATION

被引:9
作者
BRADLEY, RA [1 ]
GEORGIADIS, R [1 ]
KEVAN, SD [1 ]
RICHMOND, GL [1 ]
机构
[1] UNIV OREGON,DEPT PHYS,EUGENE,OR 97403
来源
JOURNAL OF VACUUM SCIENCE & TECHNOLOGY A-VACUUM SURFACES AND FILMS | 1992年 / 10卷 / 05期
关键词
D O I
10.1116/1.577899
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
The detailed frequency dependence of second-harmonic generation (SHG) from Ag (111) is remarkably similar for the metal/electrolyte and metal/vacuum interface. In both environments, resonant enhancement of the SHG is observed which is attributed to optical transitions at the metal surface consistent with the surface electronic band structure.
引用
收藏
页码:2996 / 3000
页数:5
相关论文
共 23 条
[1]   COMPARISON OF THE 2ND-HARMONIC RESPONSE FROM AG(111) IN UHV AND SOLUTION [J].
BRADLEY, RA ;
AREKAT, S ;
GEORGIADIS, R ;
ROBINSON, JM ;
KEVAN, SD ;
RICHMOND, GL .
CHEMICAL PHYSICS LETTERS, 1990, 168 (05) :468-472
[2]   ANISOTROPIC INTERBAND EFFECTS IN ELECTROREFLECTANCE OF AG [J].
FURTAK, TE ;
LYNCH, DW .
PHYSICAL REVIEW LETTERS, 1975, 35 (14) :960-963
[3]  
FURTAK TE, 1990, B AM PHSY SOC, V35, P218
[4]   EFFECT OF OPTICAL RESONANCES ON THE 2ND HARMONIC RESPONSE FROM AG(111) AND AG(110) IN SOLUTION [J].
GEORGIADIS, R ;
NEFF, GA ;
RICHMOND, GL .
JOURNAL OF CHEMICAL PHYSICS, 1990, 92 (07) :4623-4625
[5]   WAVELENGTH-DEPENDENT 2ND HARMONIC-GENERATION FROM AG(111) IN SOLUTION [J].
GEORGIADIS, R ;
RICHMOND, GL .
JOURNAL OF PHYSICAL CHEMISTRY, 1991, 95 (07) :2895-2899
[6]   IMAGE POTENTIAL STATES SEEN VIA 2-PHOTON PHOTOEMISSION AND 2ND HARMONIC-GENERATION [J].
GIESEN, K ;
HAGE, F ;
RIESS, HJ ;
STEINMANN, W ;
HAIGHT, R ;
BEIGANG, R ;
DREYFUS, R ;
AVOURIS, P ;
HIMPSEL, FJ .
PHYSICA SCRIPTA, 1987, 35 (04) :578-581
[7]   ELECTRONIC DISTRIBUTION AND NONLINEAR OPTICAL-RESPONSE AT THE METAL-ELECTROLYTE INTERFACE [J].
GUYOTSIONNEST, P ;
TADJEDDINE, A ;
LIEBSCH, A .
PHYSICAL REVIEW LETTERS, 1990, 64 (14) :1678-1681
[8]   OBSERVATION OF SURFACE-STATES AT THE METAL ELECTROLYTE INTERFACE BY ELECTROREFLECTANCE SPECTROSCOPY [J].
HO, KM ;
FU, CL ;
LIU, SH ;
KOLB, DM ;
PIAZZA, G .
JOURNAL OF ELECTROANALYTICAL CHEMISTRY, 1983, 150 (1-2) :235-240
[9]   A POWER-SQUARED SENSOR FOR 2-PHOTON SPECTROSCOPY AND DISPERSION OF 2ND-ORDER COHERENCE [J].
JONES, RD ;
CALLIS, PR .
JOURNAL OF APPLIED PHYSICS, 1988, 64 (09) :4301-4305
[10]   HIGH-RESOLUTION PHOTOEMISSION-STUDY OF THE ELECTRONIC-STRUCTURE OF THE NOBLE-METAL (111) SURFACES [J].
KEVAN, SD ;
GAYLORD, RH .
PHYSICAL REVIEW B, 1987, 36 (11) :5809-5818